Flexible TiO2/Au thin films with greatly enhanced photocurrents for photoelectrochemical water splitting

被引：17

作者：

Chen, Jialin ^{[1
]}

Zhang, Jiaqi ^{[1
]}

Ye, Mao ^{[2
]}

Rao, Zhenggang ^{[3
]}

Tian, Tingfang ^{[3
]}

Shu, Longlong ^{[3
]}

Lin, Peng ^{[1
]}

Zeng, Xierong ^{[1
]}

Ke, Shanming ^{[3
]}

机构：

[1] Shenzhen Univ, Coll Mat Sci & Engn, Shenzhen 518060, Guangdong, Peoples R China

[2] Southern Univ Sci & Technol, Dept Phys, Shenzhen 518055, Guangdong, Peoples R China

[3] Nanchang Univ, Sch Mat Sci & Engn, Nanchang 330031, Jiangxi, Peoples R China

来源：

JOURNAL OF ALLOYS AND COMPOUNDS | 2020年 / 815卷

基金：

中国国家自然科学基金;

关键词：

Flexibility and stability; Photoelectrochemical properties; Bilayer structure; Titanium dioxide; TITANIUM-OXIDE; NANOSTRUCTURES; HETEROJUNCTION; ABSORPTION; INSULATOR; GROWTH; SOLAR; MICA; VAN;

D O I：

10.1016/j.jallcom.2019.152471

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Photocatalysts with high flexibility and stability have become hot spots in material science and energy-related research. In this work, a TiO2/Au bilayer was developed on a flexible mica substrate for photoelectrochemical (PEC) water splitting. Due to the high temperature tolerance of mica, anatase TiO(2 )could be deposited directly on the flexible substrate. By inserting an Au layer, the photocurrent density of the TiO2/Au bilayer was 76 times higher than that of pure TiO2. Moreover, the performance of this bilayer structure has good stability for 500 bending cycles. This study provides a new research direction for the design and manufacture of flexible photoelectrochemical materials. (C) 2019 Elsevier B.V. All rights reserved.

引用

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