Electrically Pumped Polarized Exciton-Polaritons in a Halide Perovskite Microcavity

被引:22
作者
Wang, Tingting [1 ,2 ,3 ]
Zang, Zhihao [1 ,2 ,3 ]
Gao, Yuchen [1 ,2 ]
Lyu, Chao [1 ,2 ]
Gu, Pingfan [1 ,2 ]
Yao, Yige [1 ,2 ]
Peng, Kai [8 ]
Watanabe, Kenji [4 ]
Taniguchi, Takashi [5 ]
Liu, Xiaoze [6 ,7 ]
Gao, Yunan [1 ,2 ]
Bao, Wei [8 ]
Ye, Yu [1 ,2 ,3 ,9 ]
机构
[1] Peking Univ, State Key Lab Mesoscop Phys, Sch Phys, Beijing 100871, Peoples R China
[2] Peking Univ, Frontiers Sci Ctr Nanooptoelect, Sch Phys, Beijing 100871, Peoples R China
[3] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China
[4] Natl Inst Mat Sci, Res Ctr Funct Mat, Tsukuba, Ibaraki 3050044, Japan
[5] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton, Tsukuba, Ibaraki 3050044, Japan
[6] Wuhan Univ, Sch Phys & Technol, Wuhan 430072, Hubei, Peoples R China
[7] Wuhan Inst Quantum Technol, Wuhan 430206, Hubei, Peoples R China
[8] Univ Nebraska, Elect & Comp Engn, Lincoln, NE 68588 USA
[9] Peking Univ, Yangtze Delta Inst Optoelect, Nantong 226010, Jiangsu, Peoples R China
基金
美国国家科学基金会; 国家重点研发计划; 中国国家自然科学基金;
关键词
exciton-polariton; electrically pumped; perovskite; microcavity; NANOCRYSTALS; ADHESION;
D O I
10.1021/acs.nanolett.2c00906
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Recently, exciton-polaritons in lead halide perovskite microcavities have been extensively investigated to address striking phenomena such as polariton condensation and quantum emulation. However, a critical step in advancing these findings into practical applications, i.e., realizing electrically pumped perovskite polariton light-emitting devices, has not yet been presented. Here, we devise a new method to combine the device with a microcavity and report the first halide perovskite polariton light-emitting device. Specifically, the device is based on a CsPbBr3 capacitive structure, which can inject the electrons and holes from the same electrode, conducive to the formation of excitons and simultaneously maintaining the high quality of the microcavity. In addition, highly polarized polariton emissions have been demonstrated due to the optical birefringence in the CsPbBr3 microplate. This work paves the way for realizing practical polaritonic devices such as high-speed light-emitting devices for information communications and inversionless electrically pumped lasers based on perovskites.
引用
收藏
页码:5175 / 5181
页数:7
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