A Flexible All-in-One Lithium-Sulfur Battery A Flexible All-in-One Lithium-Sulfur Battery

被引:103
作者
Yao, Minjie [1 ]
Wang, Rui [1 ]
Zhao, Zifang [1 ]
Liu, Yue [1 ]
Niu, Zhiqiang [1 ]
Chen, Jun [1 ]
机构
[1] Nankai Univ, Coll Chem, Key Lab Adv Energy Mat Chem, Minist Educ, Tianjin 300071, Peoples R China
基金
中国国家自然科学基金;
关键词
carbon nanotubes; flexible; all-in-one; integrated; lithium-sulfur battery; WALLED CARBON NANOTUBES; REDUCED GRAPHENE OXIDE; SOLID-STATE; SUPERCAPACITORS; COMPOSITE; ELECTRODE; CATHODES; HYBRIDS; STORAGE; CELLS;
D O I
10.1021/acsnano.8b06936
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The recent boom in flexible and wearable electronic devices has increased the demand for flexible energy storage devices. The flexible lithium-sulfur (Li-S) battery is considered to be a promising candidate due to its high energy density and low cost. Herein, a flexible Li-S battery was fabricated based on an all-in-one integrated configuration, where a multiwalled carbon nanotubes/sulfur (MWCNTs/S) cathode, MWCNTs/manganese dioxide (MnO2) interlayer, polypropylene (PP) separator, and Li anode were integrated together by combining blade coating with vacuum evaporation methods. Each component of the all-in-one structure can be seamlessly connected with the neighboring layers. Such an optimal interfacial connection can effectively enhance electron- and/or load-transfer capacity by avoiding the relative displacement or detachment between two neighboring components at bending strain. Therefore, the flexible all-in-one Li-S batteries display fast electrochemical kinetics and have stable electrochemical performance under different bending states.
引用
收藏
页码:12503 / 12511
页数:9
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