Where air quality has been impacted by weather changes in the United States over the last 30 years?

被引:5
作者
Requia, Weeberb J. [1 ,3 ]
Coull, Brent A. [2 ]
Koutrakis, Petros [1 ]
机构
[1] Harvard Univ, Sch Publ Hlth, Dept Environm Hlth, Boston, MA 02115 USA
[2] Harvard Univ, Sch Publ Hlth, Dept Biostat, Boston, MA 02115 USA
[3] Getulio Vargas Fdn, Sch Publ Policy & Govt, Brasilia, DF, Brazil
关键词
Air pollution; Weather; Climate impact; Trend analysis; CARBON-MONOXIDE; BOOTSTRAP METHODS; OZONE; POLLUTION; CLIMATE; PM2.5; VARIABILITY; TRENDS; OXIDE; DENITRIFICATION;
D O I
10.1016/j.atmosenv.2020.117360
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Previous studies have contributed to the understanding on the impacts of weather on air pollution. Most of these investigations focused primarily on future climate scenarios, laboratory experiments, or weather trends-related air pollution at regional scale. In particular, an important limitation of the trends studies is that the estimated weather impact on air pollution may be underestimated or overestimated given that the regional scale does not capture the site-to-site variation of air pollution and weather. The primary objective of this research is to addresses this gap by quantifying weather-associated changes in air pollution at site location (air pollution sites) in the U.S between 1988 and 2018. We quantified the past weather-related increases CO, NO2, O-3, nitrate, organic carbon, silicon, sodium, sulfate, and SO2 concentration using Generalized Additive Models (GAMs). We used a framework that derives "penalties" (weather penalty, in mu g/m(3), ppm or ppb per year) for each season (warm and cold). Three pollutants presented significant results (weather penalties), including CO, NO2, and O-3. Our findings show significant spatio-temporal variation of climate impact on CO, NO2, and O-3. For example, in the warm season we estimated a total penalty over the study period for the sites with the highest penalty on CO (site in Boise, Idaho), NO2 (site in New York City), and O-3 (site in Tucson, Arizona) of 6.18 (95%CI: 0.30; 12.0) ppm, 182.04 (95%CI: 39.33; 324.72) ppb, and 0.09 (95%CI: 0.030; 0.150) ppm, respectively. In the cold season, the estimated total penalty for the sites with the highest penalty on CO (site in Los Angeles, California), NO2 (site in Washington, Pennsylvania), and O-3 (site in Decatur, Illinois) was 12.01 (95%CI: 1.50; 22.50) ppm, 285.03 (95% CI: 14.37; 555.69) ppb, and 0.066 (95%CI: -0.120; 0.030) ppm, respectively. Our results should be of interest to policy makers to create future strategies related to environmental health and climate change. Climate models typically show large variation in projections of the key variables influencing pollution, and our model based on local scale allowed us to identify statistically robust results.
引用
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页数:11
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共 51 条
  • [1] Monitoring Nitrogen Dioxide Levels in Urban Areas in Rawalpindi, Pakistan
    Ahmad, Sheikh Saeed
    Biiker, Patrick
    Emberson, Lisa
    Shabbir, Rabia
    [J]. WATER AIR AND SOIL POLLUTION, 2011, 220 (1-4) : 141 - 150
  • [2] Agriculture is a major source of NOx pollution in California
    Almaraz, Maya
    Bai, Edith
    Wang, Chao
    Trousdell, Justin
    Conley, Stephen
    Faloona, Ian
    Houlton, Benjamin Z.
    [J]. SCIENCE ADVANCES, 2018, 4 (01):
  • [3] Ozone trends and their relationship to characteristic weather patterns
    Austin, Elena
    Zanobetti, Antonella
    Coull, Brent
    Schwartz, Joel
    Gold, Diane R.
    Koutrakis, Petros
    [J]. JOURNAL OF EXPOSURE SCIENCE AND ENVIRONMENTAL EPIDEMIOLOGY, 2015, 25 (05) : 532 - 542
  • [4] Berger J.O., 2016, OBJECTIVE BAYESIAN A, DOI [10.1198/016214501753382282, DOI 10.1198/016214501753382282.]
  • [5] Plant volatiles in polluted atmospheres: stress responses and signal degradation
    Blande, James D.
    Holopainen, Jarmo K.
    Niinemets, Uelo
    [J]. PLANT CELL AND ENVIRONMENT, 2014, 37 (08) : 1892 - 1904
  • [6] Trends in U.S. Surface Humidity, 1930-2010
    Brown, Paula J.
    DeGaetano, Arthur T.
    [J]. JOURNAL OF APPLIED METEOROLOGY AND CLIMATOLOGY, 2013, 52 (01) : 147 - 163
  • [7] Simulating reactive nitrogen, carbon monoxide, and ozone in California during ARCTAS-CARB 2008 with high wildfire activity
    Cai, Chenxia
    Kulkarni, Sarika
    Zhao, Zhan
    Kaduwela, Ajith P.
    Avise, Jeremy C.
    DaMassa, John A.
    Singh, Hanwant B.
    Weinheimer, Andrew J.
    Cohen, Ronald C.
    Diskin, Glenn S.
    Wennberg, Paul
    Dibb, Jack E.
    Huey, Greg
    Wisthaler, Armin
    Jimenez, Jose L.
    Cubison, Michael J.
    [J]. ATMOSPHERIC ENVIRONMENT, 2016, 128 : 28 - 44
  • [8] A numerical study of the dependence of long-range transport of CO to a mountain station in Taiwan on synoptic weather patterns during the Southeast Asia biomass-burning season
    Cheng, Fang-Yi
    Yang, Zhih-Min
    Ou-Yang, Chang-Feng
    Ngan, Fong
    [J]. ATMOSPHERIC ENVIRONMENT, 2013, 78 : 277 - 290
  • [9] Assessment of potential improvements on regional air quality modelling related with implementation of a detailed methodology for traffic emission estimation
    Coelho, Margarida C.
    Fontes, Tania
    Bandeira, Jorge M.
    Pereira, Sergio R.
    Tchepel, Oxana
    Dias, Daniela
    Sa, Elisa
    Amorim, Jorge H.
    Borrego, Carlos
    [J]. SCIENCE OF THE TOTAL ENVIRONMENT, 2014, 470 : 127 - 137
  • [10] Imaging of molecular target modulation in oncology: Challenges of early clinical trials
    Cullinane C.
    Solomon B.
    Hicks R.J.
    [J]. Clinical and Translational Imaging, 2014, 2 (1) : 5 - 12