Attosecond spectroscopy for the investigation of ultrafast dynamics in atomic, molecular and solid-state physics

被引:90
作者
Borrego-Varillas, Rocio [1 ]
Lucchini, Matteo [1 ,2 ]
Nisoli, Mauro [1 ,2 ]
机构
[1] Consiglio Nazl Ric CNR, Inst Photon & Nanotechnol IFN, Piazza Leonardo da Vinci 32, I-20133 Milan, Italy
[2] Politecn Milan, Dept Phys, Piazza Leonardo da Vinci 32, I-20133 Milan, Italy
基金
欧洲研究理事会;
关键词
attosecond spectroscopy; femtosecond spectroscopy; atomic and molecular physics; condensed phase spectroscopy; REAL-TIME OBSERVATION; ORDER HARMONIC-GENERATION; TRANSIENT ABSORPTION-SPECTROSCOPY; X-RAY SPECTROSCOPY; CHARGE MIGRATION; ELECTRON DYNAMICS; FANO RESONANCE; PHOTOEMISSION-SPECTROSCOPY; PHOTOELECTRON-SPECTROSCOPY; ULTRAVIOLET-RADIATION;
D O I
10.1088/1361-6633/ac5e7f
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Since the first demonstration of the generation of attosecond pulses (1 as = 10(-18) s) in the extreme-ultraviolet spectral region, several measurement techniques have been introduced, at the beginning for the temporal characterization of the pulses, and immediately after for the investigation of electronic and nuclear ultrafast dynamics in atoms, molecules and solids with unprecedented temporal resolution. The attosecond spectroscopic tools established in the last two decades, together with the development of sophisticated theoretical methods for the interpretation of the experimental outcomes, allowed to unravel and investigate physical processes never observed before, such as the delay in photoemission from atoms and solids, the motion of electrons in molecules after prompt ionization which precede any notable nuclear motion, the temporal evolution of the tunneling process in dielectrics, and many others. This review focused on applications of attosecond techniques to the investigation of ultrafast processes in atoms, molecules and solids. Thanks to the introduction and ongoing developments of new spectroscopic techniques, the attosecond science is rapidly moving towards the investigation, understanding and control of coupled electron-nuclear dynamics in increasingly complex systems, with ever more accurate and complete investigation techniques. Here we will review the most common techniques presenting the latest results in atoms, molecules and solids.
引用
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页数:53
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