ZnO:Co diluted magnetic semiconductor or hybrid nanostructure for spintronics?

被引:14
作者
Golmar, F. [2 ]
Villafuerte, M. [1 ]
Mudarra Navarro, A. [3 ]
Rodriguez Torres, C. E. [3 ]
Barzola-Quiquia, J. [4 ]
Esquinazi, P. [4 ]
Heluani, S. P. [1 ]
机构
[1] Univ Nacl Tucuman, Lab Fis Solido, Dept Fis, Fac Ciencias Exactas & Tecnol,CONICET, San Miguel De Tucuman, Argentina
[2] Univ Buenos Aires, Fac Ingn, Dept Fis, Lab Ablac Laser, Buenos Aires, DF, Argentina
[3] Univ Nacl La Plata, Dept Fis IFLP, Fac Ciencias Exactas, La Plata, Buenos Aires, Argentina
[4] Univ Leipzig, Div Superconduct & Magnetism, Inst Expt Phys 2, Leipzig, Germany
关键词
FERROMAGNETISM; EXCHANGE;
D O I
10.1007/s10853-010-4710-2
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have studied the influence of intrinsic and extrinsic defects in the magnetic and electrical transport properties of Co-doped ZnO thin films. X-ray absorption measurements show that Co substitute Zn in the ZnO structure and it is in the 2+ oxidation state. Magnetization (M) measurements show that doped samples are mainly paramagnetic. From M vs. H loops measured at 5 K we found that the values of the orbital L and spin S numbers are between 1 and 1.3 for L and S = 3/2, in agreement with the representative values for isolated Co 2+. The obtained negative values of the Curie-Weiss temperatures indicate the existence of antiferromagnetic interactions between transition metal atoms.
引用
收藏
页码:6174 / 6178
页数:5
相关论文
共 13 条
[1]   Structural and magnetic properties of wurtzite CoO thin films [J].
Alaria, J. ;
Cheval, N. ;
Rode, K. ;
Venkatesan, M. ;
Coey, J. M. D. .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2008, 41 (13)
[2]  
ANDREARCZYK T, 2005, PHYS REV B, V72, P121
[3]   Donor impurity band exchange in dilute ferromagnetic oxides [J].
Coey, JMD ;
Venkatesan, M ;
Fitzgerald, CB .
NATURE MATERIALS, 2005, 4 (02) :173-179
[4]   Origin of ferromagnetism in Zn1-xCoxO from magnetization and spin-dependent magnetoresistance measurements [J].
Dietl, T. ;
Andrearczyk, T. ;
Lipinska, A. ;
Kiecana, M. ;
Tay, Maureen ;
Wu, Yihong .
PHYSICAL REVIEW B, 2007, 76 (15)
[5]   Zener model description of ferromagnetism in zinc-blende magnetic semiconductors [J].
Dietl, T ;
Ohno, H ;
Matsukura, F ;
Cibert, J ;
Ferrand, D .
SCIENCE, 2000, 287 (5455) :1019-1022
[6]   Magnetic properties of epitaxially grown semiconducting Zn1-xCoxO thin films by pulsed laser deposition [J].
Kim, JH ;
Kim, H ;
Kim, D ;
Ihm, YE ;
Choo, WK .
JOURNAL OF APPLIED PHYSICS, 2002, 92 (10) :6066-6071
[7]   Absence of intrinsic ferromagnetic interactions of isolated and paired co dopant atoms in Zn1-xCoxO with high structural perfection [J].
Ney, A. ;
Ollefs, K. ;
Ye, S. ;
Kammermeier, T. ;
Ney, V. ;
Kaspar, T. C. ;
Chambers, S. A. ;
Wilhelm, F. ;
Rogalev, A. .
PHYSICAL REVIEW LETTERS, 2008, 100 (15)
[8]   Role of defects in ferromagnetism in Zn1-xCoxO:: A hybrid density-functional study [J].
Patterson, C. H. .
PHYSICAL REVIEW B, 2006, 74 (14)
[9]   Antiferromagnetic interactions in single crystalline Zn1-xCoxO thin films [J].
Sati, P. ;
Deparis, C. ;
Morhain, C. ;
Schafer, S. ;
Stepanov, A. .
PHYSICAL REVIEW LETTERS, 2007, 98 (13)
[10]   INFLUENCE OF S-D EXCHANGE INTERACTION ON THE CONDUCTIVITY OF CD1-XMNXSE-IN IN THE WEAKLY LOCALIZED REGIME [J].
SAWICKI, M ;
DIETL, T ;
KOSSUT, J ;
IGALSON, J ;
WOJTOWICZ, T ;
PLESIEWICZ, W .
PHYSICAL REVIEW LETTERS, 1986, 56 (05) :508-511