Electron Dynamics in a Two-Dimensional Nanobubble: A Two-Level System Based on Spatial Density

被引:4
作者
Rosati, Roberto [3 ]
Lengers, Frank [1 ]
Carmesin, Christian [2 ]
Florian, Matthias [2 ]
Kuhn, Tilmann [1 ]
Jahnke, Frank [2 ]
Lorke, Michael [2 ]
Reiter, Doris E. [1 ]
机构
[1] Univ Munster, Inst Solid State Theory, D-48149 Munster, Germany
[2] Univ Bremen, Inst Theoret Phys, D-28334 Bremen, Germany
[3] Philipps Univ Marburg, Dept Phys, D-35032 Marburg, Germany
关键词
Electronic Poincare ' sphere; TMDC monolayers; nanobubbles; transport; capture; EMITTERS; OPTOELECTRONICS; EXCITONS; EMISSION; BUBBLES;
D O I
10.1021/acs.nanolett.1c02864
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Nanobubbles formed in monolayers of transition metal dichalcogenides (TMDCs) on top of a substrate feature localized potentials in which electrons can be captured. We show that the captured electronic density can exhibit a nontrivial spatiotemporal dynamics, whose movements can be mapped to states in a two-level system illustrated as points of an electronic Poincare' sphere. These states can be fully controlled, i.e, initialized and switched, by multiple electronic wave packets. Our results could be the foundation for novel implementations of quantum circuits.
引用
收藏
页码:9896 / 9902
页数:7
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