Attosecond transient absorption spooktroscopy: a ghost imaging approach to ultrafast absorption spectroscopy

被引：46

作者：

Driver, Taran ^{[1
,2
,3
]}

Li, Siqi ^{[2
,4
]}

Champenois, Elio G. ^{[1
]}

Duris, Joseph ^{[2
]}

Ratner, Daniel ^{[2
]}

Lane, Thomas J. ^{[2
]}

Rosenberger, Philipp ^{[1
,5
,6
]}

Al-Haddad, Andre ^{[7
]}

Averbukh, Vitali ^{[3
]}

Barnard, Toby ^{[3
]}

Berrah, Nora ^{[8
]}

Bostedt, Christoph ^{[7
,9
]}

Bucksbaum, Philip H. ^{[1
,4
,10
]}

Coffee, Ryan ^{[1
,2
]}

DiMauro, Louis F. ^{[11
]}

Fang, Li ^{[11
]}

Garratt, Douglas ^{[3
]}

Gatton, Averell ^{[2
]}

Guo, Zhaoheng ^{[1
,4
]}

Hartmann, Gregor ^{[12
,13
,16
]}

Haxton, Daniel ^{[14
]}

Helml, Wolfram ^{[15
]}

Huang, Zhirong ^{[2
,4
]}

LaForge, Aaron ^{[8
]}

Kamalov, Andrei ^{[1
,4
]}

Kling, Matthias F. ^{[1
,5
,6
]}

Knurr, Jonas ^{[1
]}

Lin, Ming-Fu ^{[2
]}

Lutman, Alberto A. ^{[2
]}

MacArthur, James P. ^{[2
,4
]}

Marangos, Jon P. ^{[3
]}

Nantel, Megan ^{[2
,4
]}

Natan, Adi ^{[1
]}

Obaid, Razib ^{[8
]}

O'Neal, Jordan T. ^{[1
,4
]}

Shivaram, Niranjan H. ^{[2
]}

Schori, Aviad ^{[1
]}

Walter, Peter ^{[2
]}

Wang, Anna Li ^{[1
,10
]}

Wolf, Thomas J. A. ^{[1
]}

Marinelli, Agostino ^{[2
]}

Cryan, James P. ^{[1
,2
]}

机构：

[1] SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA

[2] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA

[3] Imperial Coll London, Dept Phys, Blackett Lab, London, England

[4] Stanford Univ, Dept Phys, Stanford, CA 94305 USA

[5] Max Planck Inst Quantum Opt, Garching, Germany

[6] Ludwig Maximilians Univ Munchen, Phys Dept, Munich, Germany

[7] Paul Scherrer Inst, Villigen, Switzerland

[8] Univ Connecticut, Phys Dept, Storrs, CT USA

[9] Ecole Polytech Fed Lausanne, LUXS, Lausanne, Switzerland

[10] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA

[11] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA

[12] Univ Kassel, Inst Phys, Kassel, Germany

[13] Univ Kassel, CINSaT, Kassel, Germany

[14] KLA Tencor Corp, Milpitas, CA USA

[15] Tech Univ Dortmund, Zentrum Synchrotronstrahlung, Dortmund, Germany

[16] Helmholtz Zentrum Berlin, Berlin, Germany

来源：

PHYSICAL CHEMISTRY CHEMICAL PHYSICS | 2020年 / 22卷 / 05期

基金：

英国工程与自然科学研究理事会;

关键词：

MOLECULAR-DYNAMICS; ELECTRON DYNAMICS; RAY; GENERATION;

D O I：

10.1039/c9cp03951a

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The recent demonstration of isolated attosecond pulses from an X-ray free-electron laser (XFEL) opens the possibility for probing ultrafast electron dynamics at X-ray wavelengths. An established experimental method for probing ultrafast dynamics is X-ray transient absorption spectroscopy, where the X-ray absorption spectrum is measured by scanning the central photon energy and recording the resultant photoproducts. The spectral bandwidth inherent to attosecond pulses is wide compared to the resonant features typically probed, which generally precludes the application of this technique in the attosecond regime. In this paper we propose and demonstrate a new technique to conduct transient absorption spectroscopy with broad bandwidth attosecond pulses with the aid of ghost imaging, recovering sub-bandwidth resolution in photoproduct-based absorption measurements.

引用

页码：2704 / 2712

页数：9

共 43 条

[1] Supercontinuum spectral-domain ghost imaging [J].

Amiot, Caroline ;

Ryczkowski, Piotr ;

Friberg, Ari T. ;

Dudley, John M. ;

Genty, Goery .

OPTICS LETTERS, 2018, 43 (20) :5025-5028

[2]

[Anonymous], FOUND TRENDS MACH LE

[3] Femtosecond x-ray spectroscopy of an electrocyclic ring-opening reaction [J].

Attar, Andrew R. ;

Bhattacherjee, Aditi ;

Pemmaraju, C. D. ;

Schnorr, Kirsten ;

Closser, Kristina D. ;

Prendergast, David ;

Leone, Stephen R. .

SCIENCE, 2017, 356 (6333) :54-58

[4] K- and L-edge X-ray absorption spectroscopy (XAS) and resonant inelastic X-ray scattering (RIXS) determination of differential orbital covalency (DOC) of transition metal sites [J].

Baker, Michael L. ;

Mara, Michael W. ;

Yan, James J. ;

Hodgson, Keith O. ;

Hedman, Britt ;

Solomon, Edward I. .

COORDINATION CHEMISTRY REVIEWS, 2017, 345 :182-208

[5] Probing ultrafast dynamics with attosecond transient absorption [J].

Beck, Annelise R. ;

Neumark, Daniel M. ;

Leone, Stephen R. .

CHEMICAL PHYSICS LETTERS, 2015, 624 :119-130

[6] A perspective for investigating photo-induced molecular dynamics from within with femtosecond free electron lasers [J].

Berrah, Nora .

PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2017, 19 (30) :19536-19544

[7] Ultrafast X-ray absorption spectroscopy [J].

Bressler, C ;

Chergui, M .

CHEMICAL REVIEWS, 2004, 104 (04) :1781-1812

[8] Ultrafast electron dynamics in phenylalanine initiated by attosecond pulses [J].

Calegari, F. ;

Ayuso, D. ;

Trabattoni, A. ;

Belshaw, L. ;

De Camillis, S. ;

Anumula, S. ;

Frassetto, F. ;

Poletto, L. ;

Palacios, A. ;

Decleva, P. ;

Greenwood, J. B. ;

Martin, F. ;

Nisoli, M. .

SCIENCE, 2014, 346 (6207) :336-339

[9]

Champenois Elio., 2017, pbasex abel transform inversion without polar rebinning

[10] The generation, characterization and applications of broadband isolated attosecond pulses [J].

Chini, Michael ;

Zhao, Kun ;

Chang, Zenghu .

NATURE PHOTONICS, 2014, 8 (03) :178-186

← 1 2 3 4 5 →