Detection of vibrationally excited O2 in the active medium of a chemical oxygen-iodine laser

被引:12
作者
Azyazov, VN [1 ]
Antonov, IO [1 ]
Pichugin, SY [1 ]
Safonov, VS [1 ]
Svistum, MI [1 ]
Ufimtsev, NI [1 ]
机构
[1] PN Lebedev Phys Inst, Samara 443011, Russia
关键词
D O I
10.1070/QE2003v033n09ABEH002504
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
The presence of vibrationally excited oxygen in the active medium of a chemical oxygen - iodine laser is discovered using the emission technique. Using the analysis of the luminescence spectra of oxygen molecules on O 2(b1 Σg+, v = i) → O 2(X3 Σg-, v′ = i) (i = 0, 1, 2) electronic vibrational-rotational transitions, it is shown that ∼ 22% of O2(b1 Σg+) molecules are at the first vibrational level and ∼ 10% are at the second one. Moreover, due to the fast EE energy exchange, a mean number of vibrational quanta per one molecule in each of the O2(X3 Σ g-), O2(a1Δg) and O2(b1 Σg+ components is approximately the same and amounts to 30%-40%.
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页码:811 / 816
页数:6
相关论文
共 28 条
[21]  
KALOGERAKIS KS, 2001, EOS T AGU, V82
[22]  
Komissarov AV, 2000, PROC SPIE, V4184, P7
[23]  
Krupenie, 1972, J PHYS CHEM REF DATA, V1, P423, DOI DOI 10.1063/1.3253101
[24]   COLLISIONAL DEACTIVATION OF VIBRATIONALLY EXCITED SINGLET MOLECULAR-OXYGEN [J].
PARKER, JG ;
RITKE, DN .
JOURNAL OF CHEMICAL PHYSICS, 1973, 59 (07) :3713-3722
[25]   ENERGY POOLING REACTION 2O2(DELTA-1G) -] O2(SIGMA-3G-) + O2(SIGMA-1G+) - FORMATION, RELAXATION, AND QUENCHING OF VIBRATIONALLY EXCITED O2(SIGMA-1G+) [J].
SCHURATH, U .
JOURNAL OF PHOTOCHEMISTRY, 1975, 4 (03) :215-226
[26]   ENERGY-TRANSFER IN QUENCHING OF SINGLET MOLECULAR-OXYGEN .3. APPLICATION OF STATISTICAL-THEORY [J].
THOMAS, RGO ;
THRUSH, BA .
PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES, 1977, 356 (1686) :307-314
[27]   ENERGY-TRANSFER IN QUENCHING OF SINGLET MOLECULAR-OXYGEN .2. RATES OF FORMATION AND QUENCHING OF VIBRATIONALLY EXCITED MOLECULES [J].
THOMAS, RGO ;
THRUSH, BA .
PROCEEDINGS OF THE ROYAL SOCIETY OF LONDON SERIES A-MATHEMATICAL AND PHYSICAL SCIENCES, 1977, 356 (1686) :295-306
[28]   DETECTION OF VIBRATIONALLY EXCITED I-2 IN THE IODINE DISSOCIATION REGION OF CHEMICAL OXYGEN IODINE LASERS [J].
VANBENTHEM, MH ;
DAVIS, SJ .
JOURNAL OF PHYSICAL CHEMISTRY, 1986, 90 (05) :902-905