Enhancement in external quantum efficiency of light-emitting diode based on colloidal silicon nanocrystals

被引:4
作者
Hao, Huilian [1 ]
Zhao, Yue [1 ]
Song, Tianliang [1 ]
Wang, Xu [1 ]
Li, Changwang [1 ]
Li, Wenyao [1 ]
Shen, Wenzhong [2 ,3 ]
机构
[1] Shanghai Univ Engn Sci, Coll Mat Engn, 333 Long Teng Rd, Shanghai 201620, Peoples R China
[2] Shanghai Jiao Tong Univ, Inst Solar Energy, Dept Phys & Astron, 800 Dong Chuan Rd, Shanghai 200240, Peoples R China
[3] Shanghai Jiao Tong Univ, Key Lab Artificial Struct & Quantum Control, Dept Phys & Astron, Minist Educ, 800 Dong Chuan Rd, Shanghai 200240, Peoples R China
基金
英国工程与自然科学研究理事会;
关键词
colloidal silicon nanocrystals; light-emitting diode; electroluminescence; charge transport; SI NANOCRYSTALS; DOTS; PHOTOLUMINESCENCE; CONFINEMENT; PERFORMANCE;
D O I
10.1088/1361-6528/ac2ac1
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Herein, we report an enhanced red emission from colloidal silicon nanocrystals (c-Si NCs) solution-processed light-emitting diode. c-Si NCs were synthesized by facile femtosecond laser ablation. Based on the structural characterization and opto-electrics properties analysis, both photoluminescence and electroluminescence arise from the radiative recombination of carriers due to quantum confined effect. The optical power density and highest external quantum efficiency have been obtained to be 0.79 mW cm(-2) and similar to 6.6%, respectively. These results indicate that Si NCs are very attractive as a potential optical source for future integrated chips.
引用
收藏
页数:6
相关论文
共 33 条
[1]   High-Efficiency Silicon Nanocrystal Light-Emitting Devices [J].
Cheng, Kai-Yuan ;
Anthony, Rebecca ;
Kortshagen, Uwe R. ;
Holmes, Russell J. .
NANO LETTERS, 2011, 11 (05) :1952-1956
[2]   Hybrid Silicon Nanocrystal-Organic Light-Emitting Devices for Infrared Electroluminescence [J].
Cheng, Kai-Yuan ;
Anthony, Rebecca ;
Kortshagen, Uwe R. ;
Holmes, Russell J. .
NANO LETTERS, 2010, 10 (04) :1154-1157
[3]  
Chukwuocha E.O., 2012, WORLD J CONDENS MAT, V2, P96, DOI DOI 10.4236/WJCMP.2012.22017
[4]   Solution-processed, high-performance light-emitting diodes based on quantum dots [J].
Dai, Xingliang ;
Zhang, Zhenxing ;
Jin, Yizheng ;
Niu, Yuan ;
Cao, Hujia ;
Liang, Xiaoyong ;
Chen, Liwei ;
Wang, Jianpu ;
Peng, Xiaogang .
NATURE, 2014, 515 (7525) :96-99
[5]   Size vs Surface: Tuning the Photoluminescence of Freestanding Silicon Nanocrystals Across the Visible Spectrum via Surface Groups [J].
Dasog, Mita ;
De los Reyes, Glenda B. ;
Titova, Lyubov V. ;
Hegmann, Frank A. ;
Veinot, Jonathan G. C. .
ACS NANO, 2014, 8 (09) :9636-9648
[6]   Enhancing the electroluminescence efficiency of Si NC/SiO2 superlattice-based light-emitting diodes through hydrogen ion beam treatment [J].
Fu, Sheng-Wen ;
Chen, Hui-Ju ;
Wu, Hsuan-Ta ;
Chen, Shao-Ping ;
Shih, Chuan-Feng .
NANOSCALE, 2016, 8 (13) :7155-7162
[7]   Hybrid White Light Emitting Diode Based on Silicon Nanocrystals [J].
Ghosh, Batu ;
Masuda, Yoshitake ;
Wakayama, Yutaka ;
Imanaka, Yasutaka ;
Inoue, Jun-ichi ;
Hashi, Kenjiro ;
Deguchi, Kenzo ;
Yamada, Hideto ;
Sakka, Yoshio ;
Ohki, Shinobu ;
Shimizu, Tadashi ;
Shirahata, Naoto .
ADVANCED FUNCTIONAL MATERIALS, 2014, 24 (45) :7151-7160
[8]   Luminescent Colloidal Dispersion of Silicon Quantum Dots from Microwave Plasma Synthesis: Exploring the Photoluminescence Behavior Across the Visible Spectrum [J].
Gupta, Anoop ;
Swihart, Mark T. ;
Wiggers, Hartmut .
ADVANCED FUNCTIONAL MATERIALS, 2009, 19 (05) :696-703
[9]   Origin of blue photoluminescence from colloidal silicon nanocrystals fabricated by femtosecond laser ablation in solution [J].
Hao, H. L. ;
Wu, W. S. ;
Zhang, Y. ;
Wu, L. K. ;
Shen, W. Z. .
NANOTECHNOLOGY, 2016, 27 (32)
[10]   Origin of visible luminescence in hydrogenated amorphous silicon nitride [J].
Hao, H. L. ;
Wu, L. K. ;
Shen, W. Z. ;
Dekkers, H. F. W. .
APPLIED PHYSICS LETTERS, 2007, 91 (20)