Sensitivity of the glass transition and melting in a metal-organic framework to ligand chemistry

被引：9

作者：

Madsen, Rasmus S. K. ^{[1
]}

Sarkar, Sounak ^{[2
]}

Iversen, Bo Brummerstedt ^{[2
]}

Yue, Yuanzheng ^{[1
]}

机构：

[1] Aalbrog Univ, Dept Chem & Biosci, DK-9220 Aalborg, Denmark

[2] Aarhus Univ, Dept Chem, DK-8000 Aarhus, Denmark

来源：

CHEMICAL COMMUNICATIONS | 2022年 / 58卷 / 06期

关键词：

LIQUID;

D O I：

10.1039/d1cc03541j

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The effect of substituting linkers with electron-donating moieties for part of the conventional ones on the melting and glass transition behaviours of ZIF-62 was investigated by calorimetry and X-ray diffraction. Specifically, substituting 5,6-dimethylbenzimidazole for benzimidazole in ZIF-62 increases both T-m and T-g. The structural origin of this effect was explained.

引用

页码：823 / 826

页数：4

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