Recent progresses and remaining issues on the ultrathin catalyst layer design strategy for high-performance proton exchange membrane fuel cell with further reduced Pt loadings: A review

被引:37
作者
Deng, Xiang [1 ,2 ,3 ]
Huang, Chao [1 ,2 ]
Pei, Xiaodong [1 ,2 ]
Hu, Bin [3 ]
Zhou, Wei [3 ]
机构
[1] Sinosteel Nanjing Adv Mat Res Inst Co Ltd, Nanjing 211100, Peoples R China
[2] Sinosteel New Mat Co Ltd, Maanshan 243000, Peoples R China
[3] Nanjing Tech Univ, Coll Chem Engn, State Key Lab Mat Oriented Chem Engn, Nanjing 211816, Peoples R China
关键词
Ultrathin catalyst layer; Reduced Pt loading; Layer design strategy; PEMFC; OXYGEN-REDUCTION; CATHODE CATALYSTS; NANOTUBE ARRAYS; BIPOLAR PLATES; WATER-BALANCE; PLATINUM; ELECTRODE; TRANSPORT; PEMFC; ELECTROCATALYSTS;
D O I
10.1016/j.ijhydene.2021.10.141
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This study presents a detailed review on the ultrathin catalyst layer (UTCL) design strategy for high-performance proton exchange membrane fuel cell (PEMFC). Specifically, the motivation towards the further reduced Pt loadings by applying the UTCL electrode design is firstly introduced from both the historical and mechanism deductions. Then, the recent developments on the UTCL designs belonging to different classifications are summarized with their respective merits. In particular, the critical issues remained on these ultra-thin, low Pt-loaded electrodes are proposed with alternative solutions. Finally, the whole review is concluded with the perspectives on the possible future directions settling the remaining challenges. (c) 2021 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:1529 / 1542
页数:14
相关论文
共 101 条
[61]   Investigation of hot pressing parameters for manufacture of catalyst-coated membrane electrode (CCME) for polymer electrolyte membrane fuel cells by response surface method [J].
Roudbari, Mohsen Najafi ;
Ojani, Reza ;
Raoof, Jahan Bakhsh .
ENERGY, 2017, 140 :794-803
[62]   Atomic Layer Deposition of Pt Nanoelectrode Array for Polymer Electrolyte Fuel Cells [J].
Sabarirajan, Dinesh C. ;
George, Thomas Y. ;
Vlahakis, James ;
White, Robert D. ;
Zenyuk, Iryna V. .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2019, 166 (07) :F3081-F3088
[63]   Review on the Macro-Transport Processes Theory for Irregular Pores able to Perform Catalytic Reactions [J].
Santamaria-Holek, Ivan ;
Hernandez, Saul I. ;
Garcia-Alcantara, Consuelo ;
Ledesma-Duran, Aldo .
CATALYSTS, 2019, 9 (03)
[64]   Planar polymer electrolyte membrane fuel cells: powering portable devices from hydrogen [J].
Sapkota, Prabal ;
Boyer, Cyrille ;
Dutta, Rukmi ;
Cazorla, Claudio ;
Aguey-Zinsou, Kondo-Francois .
SUSTAINABLE ENERGY & FUELS, 2020, 4 (02) :439-468
[65]   Exploration of significant influences of the operating conditions on the local O2 transport in proton exchange membrane fuel cells (PEMFCs) [J].
Shen, Shuiyun ;
Cheng, Xiaojing ;
Wang, Chao ;
Yan, Xiaohui ;
Ke, Changchun ;
Yin, Jiewei ;
Zhang, Junliang .
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2017, 19 (38) :26221-26229
[66]   Ultrathin nanoporous metal electrodes facilitate high proton conduction for low-Pt PEMFCs [J].
Shi, Shuai ;
Wen, Xianglong ;
Sang, Qinqin ;
Yin, Shuai ;
Wang, Kaili ;
Zhang, Jian ;
Hu, Min ;
Yin, Huiming ;
He, Jia ;
Ding, Yi .
NANO RESEARCH, 2021, 14 (08) :2681-2688
[67]   Ultra-low loading Pt-sputtered gas diffusion electrodes for oxygen reduction reaction [J].
Sievers, Gustav ;
Vidakovic-Koch, Tanja ;
Walter, Christian ;
Steffen, Florian ;
Jakubith, Sven ;
Kruth, Angela ;
Hermsdorf, Dana ;
Sundmacher, Kai ;
Brueser, Volker .
JOURNAL OF APPLIED ELECTROCHEMISTRY, 2018, 48 (02) :221-232
[68]   Optimization studies of a polymer electrolyte membrane fuel cell with multiple catalyst layers [J].
Srinivasarao, Modekurti ;
Bhattacharyya, Debangsu ;
Rengaswamy, Raghunathan .
JOURNAL OF POWER SOURCES, 2012, 206 :197-203
[69]   Anode-Design Strategies for Improved Performance of Polymer-Electrolyte Fuel Cells with Ultra-Thin Electrodes [J].
Steinbach, Andrew J. ;
Allen, Jeffrey S. ;
Borup, Rodney L. ;
Hussey, Daniel S. ;
Jacobson, David L. ;
Komlev, Andrei ;
Kwong, Anthony ;
MacDonald, James ;
Mukundan, Rangachary ;
Pejsa, Matt J. ;
Roos, Michael ;
Santamaria, Anthony D. ;
Sieracki, James M. ;
Spernjak, Dusan ;
Zenyuk, Iryna V. ;
Weber, Adam Z. .
JOULE, 2018, 2 (07) :1297-1312
[70]   Controlling Pt loading and carbon matrix thickness for a high performance Pt-nanowire catalyst layer in PEMFCs [J].
Su, Kaihua ;
Sui, Sheng ;
Yao, Xianyong ;
Wei, Zhaoxu ;
Zhang, Junliang ;
Du, Shangfeng .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2014, 39 (07) :3397-3403