Recent progresses and remaining issues on the ultrathin catalyst layer design strategy for high-performance proton exchange membrane fuel cell with further reduced Pt loadings: A review

被引:31
|
作者
Deng, Xiang [1 ,2 ,3 ]
Huang, Chao [1 ,2 ]
Pei, Xiaodong [1 ,2 ]
Hu, Bin [3 ]
Zhou, Wei [3 ]
机构
[1] Sinosteel Nanjing Adv Mat Res Inst Co Ltd, Nanjing 211100, Peoples R China
[2] Sinosteel New Mat Co Ltd, Maanshan 243000, Peoples R China
[3] Nanjing Tech Univ, Coll Chem Engn, State Key Lab Mat Oriented Chem Engn, Nanjing 211816, Peoples R China
关键词
Ultrathin catalyst layer; Reduced Pt loading; Layer design strategy; PEMFC; OXYGEN-REDUCTION; CATHODE CATALYSTS; NANOTUBE ARRAYS; BIPOLAR PLATES; WATER-BALANCE; PLATINUM; ELECTRODE; TRANSPORT; PEMFC; ELECTROCATALYSTS;
D O I
10.1016/j.ijhydene.2021.10.141
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This study presents a detailed review on the ultrathin catalyst layer (UTCL) design strategy for high-performance proton exchange membrane fuel cell (PEMFC). Specifically, the motivation towards the further reduced Pt loadings by applying the UTCL electrode design is firstly introduced from both the historical and mechanism deductions. Then, the recent developments on the UTCL designs belonging to different classifications are summarized with their respective merits. In particular, the critical issues remained on these ultra-thin, low Pt-loaded electrodes are proposed with alternative solutions. Finally, the whole review is concluded with the perspectives on the possible future directions settling the remaining challenges. (c) 2021 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:1529 / 1542
页数:14
相关论文
共 50 条
  • [1] Particle Size Effects of Pt Nanocatalyst in the Catalyst Layer of Proton Exchange Membrane Fuel Cell
    Wang Aili
    Sun Yu
    Liang Zhixiu
    Chen Shengli
    ACTA CHIMICA SINICA, 2009, 67 (22) : 2554 - 2558
  • [2] Performance improvement of ultra-low Pt proton exchange membrane fuel cell by catalyst layer structure optimization
    Xi, Jinyan
    Meng, Kang
    Li, Ying
    Wang, Meng
    Liao, Qiang
    Wei, Zidong
    Shao, Minhua
    Wang, Jianchuan
    CHINESE JOURNAL OF CHEMICAL ENGINEERING, 2022, 41 : 473 - 479
  • [3] High Performance Carbon Supported Palladium Catalyst in Anodes of Proton Exchange Membrane Fuel Cell
    Bonifacio, Rafael Nogueira
    Neto, Almir Oliveira
    Linardi, Marcelo
    INTERNATIONAL JOURNAL OF ELECTROCHEMICAL SCIENCE, 2013, 8 (01): : 159 - 167
  • [4] High-performance proton exchange membrane fuel cell with ultra-low loading Pt on vertically aligned carbon nanotubes as integrated catalyst layer
    Meng, Qing Hao
    Hao, Chao
    Yan, Bowen
    Yang, Bin
    Liu, Jia
    Shen, Pei Kang
    Tian, Zhi Qun
    JOURNAL OF ENERGY CHEMISTRY, 2022, 71 : 497 - 506
  • [5] Proton Exchange Membrane Fuel Cell Catalyst Layer Degradation Mechanisms: A Succinct Review
    Okonkwo, Paul C.
    CATALYSTS, 2025, 15 (01)
  • [6] High-performance long-term driving proton exchange membrane fuel cell implemented with chemically ordered Pt-based alloy catalyst at ultra-low Pt loading
    Kim, Youngkwang
    Bae, Hyo Eun
    Lee, Dohyeon
    Kim, Jeongwoo
    Lee, Eunjik
    Oh, Songi
    Jang, Ji-Hoon
    Cho, Yong-Hun
    Karuppannan, Mohanraju
    Sung, Yung-Eun
    Lim, Taeho
    Kwon, Oh Joong
    JOURNAL OF POWER SOURCES, 2022, 533
  • [7] Gradient Hydrophobic Microporous Layer for High-Performance Proton-Exchange Membrane Fuel Cells
    Wang, Wei
    Guo, Jie
    Gu, Tianyi
    Shi, Ruhua
    Wei, Xian
    Zhang, Qian
    Wang, Haibo
    Yang, Ruizhi
    ENERGY & FUELS, 2024, 38 (03) : 2368 - 2376
  • [8] Microscale structure optimization of catalyst layer for comprehensive performance enhancement in proton exchange membrane fuel cell
    Zhou, Yu
    Wu, Mingyang
    Meng, Kai
    Liu, Yurong
    Rao, Peng
    Wu, Xiao
    Huang, Shuyi
    Li, Ke
    Zheng, Chongwei
    Wu, Daoxiong
    Deng, Peilin
    Li, Jing
    Tian, Xinlong
    Kang, Zhenye
    ENERGY, 2024, 301
  • [9] Effect of Adding Zinc Oxide Particles to the Anode Catalyst Layer on the Performance of a Proton-Exchange Membrane Fuel Cell
    Fang, Sheng-Yu
    Teoh, Lay Gaik
    Huang, Rong-Hsin
    Chao, Wen-Kai
    Lin, Tien-Jen
    Yang, Kai-Chun
    Hsueh, Kan-Lin
    Shieu, Fuh-Sheng
    JOURNAL OF ELECTRONIC MATERIALS, 2014, 43 (09) : 3601 - 3610
  • [10] A unified catalyst layer design classification criterion on proton exchange membrane fuel cell performance based on a modified agglomerate model
    Wang, N.
    Qu, Z. G.
    Jiang, Z. Y.
    Zhang, G. B.
    CHEMICAL ENGINEERING JOURNAL, 2022, 447