Recent Advances in 3D Graphene Architectures and Their Composites for Energy Storage Applications

被引：117

作者：

Wang, Zhijie ^{[1
]}

Gao, Hong ^{[1
]}

Zhang, Qing ^{[1
]}

Liu, Yuqing ^{[2
]}

Chen, Jun ^{[2
]}

Guo, Zaiping ^{[1
,3
]}

机构：

[1] Univ Wollongong, AIIM, ISEM, Wollongong, NSW 2522, Australia

[2] Univ Wollongong, AIIM, IPRI, ARC Ctr Excellence Electromat Sci, Wollongong, NSW 2522, Australia

[3] Univ Wollongong, Fac Engn & Informat Sci, Sch Mech Mat Mechatron & Biomed Engn, Wollongong, NSW 2522, Australia

来源：

SMALL | 2019年 / 15卷 / 03期

基金：

澳大利亚研究理事会;

关键词：

3D graphene architectures; electrodes; energy storage; hybrid structures; NITROGEN-DOPED GRAPHENE; PERFORMANCE LI-ION; LITHIUM-ION; 3-DIMENSIONAL GRAPHENE; AEROGEL COMPOSITES; HIGH-CAPACITY; ELECTROCHEMICAL PROPERTIES; HIERARCHICAL STRUCTURE; FREESTANDING CATHODE; CHEMICAL-REDUCTION;

D O I：

10.1002/smll.201803858

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Graphene is widely applied as an electrode material in energy storage fields. However, the strong pi-pi interaction between graphene layers and the stacking issues lead to a great loss of electrochemically active surface area, damaging the performance of graphene electrodes. Developing 3D graphene architectures that are constructed of graphene sheet subunits is an effective strategy to solve this problem. The graphene architectures can be directly utilized as binder-free electrodes for energy storage devices. Furthermore, they can be used as a matrix to support active materials and further improve their electrochemical performance. Here, recent advances in synthesizing 3D graphene architectures and their composites as well as their application in different energy storage devices, including various battery systems and supercapacitors are reviewed. In addition, their challenges for application at the current stage are discussed and future development prospects are indicated.

引用

页数：21

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