ZIF-8-Derived Hollow Carbon for Efficient Adsorption of Antibiotics

被引：69

作者：

Tang, Hongmei ^{[1
]}

Li, Wenyao ^{[1
]}

Jiang, Haishun ^{[1
]}

Lin, Runjia ^{[2
]}

Wang, Zhe ^{[1
]}

Wu, Jianghong ^{[3
]}

He, Guanjie ^{[2
]}

Shearing, Paul Robert ^{[2
]}

Brett, Dan John Leslie ^{[2
]}

机构：

[1] Shanghai Univ Engn Sci, Sch Mat Engn, Shanghai 201620, Peoples R China

[2] UCL, Dept Chem Engn, Electrochem Innovat Lab, London WC1E 7JE, England

[3] Shenzhen Technol Univ, Coll Hlth Sci & Environm Engn, Shenzhen 518118, Peoples R China

来源：

NANOMATERIALS | 2019年 / 9卷 / 01期

基金：

中国国家自然科学基金; 英国工程与自然科学研究理事会; 英国科学技术设施理事会;

关键词：

ZIF-8; hollow carbon; antibiotics; adsorbent; OFLOXACIN SORPTION; TETRACYCLINE; GRAPHENE; REMOVAL; WATER; BIOCHAR;

D O I：

10.3390/nano9010117

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The harmful nature of high concentrations of antibiotics to humans and animals requires the urgent development of novel materials and techniques for their absorption. In this work, CTAB (Cetyltrimethyl Ammonium Bromide)-assisted synthesis of ZIF-8 (zeolitic imidazolate framework)-derived hollow carbon (ZHC) was designed, prepared, and used as a high-performance adsorbent, and further evaluated by Langmuir and Freundlich isothermal adsorption experiments, dynamic analysis, as well as theoretical calculation. The maximum capacities of ZHC for adsorbing tetracycline (TC), norfloxacin (NFO), and levofloxacin (OFO) are 267.3, 125.6, and 227.8 mg g(-)(1), respectively, which delivers superior adsorptive performance when compared to widely studied inorganic adsorbates. The design concept of ZIF-8-derived hollow carbon material provides guidance and insights for the efficient adsorbent of environmental antibiotics.

引用

页数：9

共 27 条

[1] Neodymium embedded ordered mesoporous carbon (OMC) for enhanced adsorption of sunset yellow: Characterizations, adsorption study and adsorption mechanism [J].

Ahmad, Zaki Uddin ;

Yao, Lunguang ;

Wang, Jin ;

Gang, Daniel Dianchen ;

Islam, Fahrin ;

Lian, Qiyu ;

Zappi, Mark E. .

CHEMICAL ENGINEERING JOURNAL, 2019, 359 :814-826

[2] A new family of carbon materials: synthesis of MOF-derived nanoporous carbons and their promising applications [J].

Chaikittisilp, Watcharop ;

Ariga, Katsuhiko ;

Yamauchi, Yusuke .

JOURNAL OF MATERIALS CHEMISTRY A, 2013, 1 (01) :14-19

[3] Synthesis of novel microporous nanocomposites of ZIF-8 on multiwalled carbon nanotubes for adsorptive removing benzoic acid from water [J].

Dai, Juan ;

Xiao, Xin ;

Duan, Suxia ;

Liu, Jing ;

He, Jing ;

Lei, Jiandu ;

Wang, Luying .

CHEMICAL ENGINEERING JOURNAL, 2018, 331 :64-74

[4]

Freundlich H, 1906, Z PHYS CHEM-STOCH VE, V57, P385

[5] Review of second-order models for adsorption systems [J].

Ho, Yuh-Shan .

JOURNAL OF HAZARDOUS MATERIALS, 2006, 136 (03) :681-689

[6] Platinum-Free Counter Electrode Comprised of Metal-Organic-Framework (MOF)-Derived Cobalt Sulfide Nanoparticles for Efficient Dye-Sensitized Solar Cells (DSSCs) [J].

Hsu, Shao-Hui ;

Li, Chun-Ting ;

Chien, Heng-Ta ;

Salunkhe, Rahul R. ;

Suzuki, Norihiro ;

Yamauchi, Yusuke ;

Ho, Kuo-Chuan ;

Wu, Kevin C. -W. .

SCIENTIFIC REPORTS, 2014, 4

[7] Effects of metal ions and pH on ofloxacin sorption to cassava residue-derived biochar [J].

Huang, Peng ;

Ge, Chengjun ;

Feng, Dan ;

Yu, Huamei ;

Luo, Jiwei ;

Li, Jiatong ;

Strong, P. J. ;

Sarmah, Ajit K. ;

Bolan, Nanthi S. ;

Wang, Hailong .

SCIENCE OF THE TOTAL ENVIRONMENT, 2018, 616 :1384-1391

[8] THE ADSORPTION OF GASES ON PLANE SURFACES OF GLASS, MICA AND PLATINUM. [J].

Langmuir, Irving .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1918, 40 :1361-1403

[9] Enhanced adsorption capacity of ultralong hydrogen titanate nanobelts for antibiotics [J].

Li, Wenyao ;

Wang, Jingru ;

He, Guanjie ;

Yu, Li ;

Noor, Nuruzzaman ;

Sun, Yangang ;

Zhou, Xiying ;

Hu, Junqing ;

Parkin, Ivan P. .

JOURNAL OF MATERIALS CHEMISTRY A, 2017, 5 (09) :4352-4358

[10] Effective Removal of Tetracycline Antibiotics from Water using Hybrid Carbon Membranes [J].

Liu, Ming-kai ;

Liu, Ying-ya ;

Bao, Dan-dan ;

Zhu, Gen ;

Yang, Guo-hai ;

Geng, Jun-feng ;

Li, Hai-tao .

SCIENTIFIC REPORTS, 2017, 7

← 1 2 3 →