Role of anthropogenic aerosols in affecting different-grade precipitation over eastern China: A case study

被引:9
作者
Shao, Tianbin [1 ]
Liu, Yuzhi [1 ,2 ]
Wang, Renruoyu [1 ]
Zhu, Qingzhe [1 ]
Tan, Ziyuan [1 ]
Luo, Run [1 ]
机构
[1] Lanzhou Univ, Coll Atmospher Sci, Key Lab Semiarid Climate Change, Minist Educ, Lanzhou 730000, Peoples R China
[2] Lanzhou Univ, Collaborat Innovat Ctr Western Ecol Safety, Lanzhou 730000, Peoples R China
基金
中国国家自然科学基金;
关键词
Anthropogenic aerosols; Precipitation; Cloud; WRF-Chem; OPTICAL-PROPERTIES; CLOUD MICROPHYSICS; AIR-POLLUTION; CLIMATE; MODEL; IMPACT; SMOKE; DUST; STORM;
D O I
10.1016/j.scitotenv.2021.150886
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Atmospheric aerosols play an important role in affecting clouds and precipitation by serving as condensation/ice nuclei. However, how to quantify the contribution of anthropogenic aerosols to the alteration of clouds and precipitation remains unknown. In this study, using a Weather Research and Forecasting-Chemistry (WRF-Chem) model, we quantified the impacts of anthropogenic aerosols on cloud water properties under different precipitation grades during a single rainfall event over eastern China. The results of this study show that anthropogenic aerosols have varying effects on hourly precipitation with heavy (greater than 1.04 mm/h), moderate (0.41-1.04 mm/h), and light (less than 0.41 mm/h) grades. Due to the presence of anthropogenic aerosols, heavy precipitation is intensified by 70.96%; however, moderate and light precipitation is further weakened by 24.87% and 86.43%, respectively. For heavy precipitation, the addition of anthropogenic aerosols induces an enhancement in upward motion, increases the cloud water path and effective radius through the aerosol radiation interaction (ARI) effect, which is the main reason for the intensification of heavy-grade precipitation. In addition, the weakened upward motion and decreased ice water path caused by ARI and aerosol-cloud interaction (ACI) effects play common roles in reducing moderate and light precipitation. Studying anthropogenic aerosols' impacts on precipitation is of great importance for understanding the influence of anthropogenic pollution on the weather and climate and even for promoting precipitation forecasting and prediction. (c) 2021 Elsevier B.V. All rights reserved.
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页数:11
相关论文
共 62 条
  • [1] AEROSOLS, CLOUD MICROPHYSICS, AND FRACTIONAL CLOUDINESS
    ALBRECHT, BA
    [J]. SCIENCE, 1989, 245 (4923) : 1227 - 1230
  • [2] [Anonymous], 2013, CLOUDS AND AEROSOLS
  • [3] Aerosol-radiation-cloud interactions in a regional coupled model: the effects of convective parameterisation and resolution
    Archer-Nicholls, Scott
    Lowe, Douglas
    Schultz, David M.
    McFiggans, Gordon
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2016, 16 (09) : 5573 - 5594
  • [4] Anthropogenic Aerosols and the Weakening of the South Asian Summer Monsoon
    Bollasina, Massimo A.
    Ming, Yi
    Ramaswamy, V.
    [J]. SCIENCE, 2011, 334 (6055) : 502 - 505
  • [5] Bounding the role of black carbon in the climate system: A scientific assessment
    Bond, T. C.
    Doherty, S. J.
    Fahey, D. W.
    Forster, P. M.
    Berntsen, T.
    DeAngelo, B. J.
    Flanner, M. G.
    Ghan, S.
    Kaercher, B.
    Koch, D.
    Kinne, S.
    Kondo, Y.
    Quinn, P. K.
    Sarofim, M. C.
    Schultz, M. G.
    Schulz, M.
    Venkataraman, C.
    Zhang, H.
    Zhang, S.
    Bellouin, N.
    Guttikunda, S. K.
    Hopke, P. K.
    Jacobson, M. Z.
    Kaiser, J. W.
    Klimont, Z.
    Lohmann, U.
    Schwarz, J. P.
    Shindell, D.
    Storelvmo, T.
    Warren, S. G.
    Zender, C. S.
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2013, 118 (11) : 5380 - 5552
  • [6] Coupling aerosol-cloud-radiative processes in the WRF-Chem model: Investigating the radiative impact of elevated point sources
    Chapman, E. G.
    Gustafson, W. I., Jr.
    Easter, R. C.
    Barnard, J. C.
    Ghan, S. J.
    Pekour, M. S.
    Fast, J. D.
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2009, 9 (03) : 945 - 964
  • [7] CLIMATE FORCING BY ANTHROPOGENIC AEROSOLS
    CHARLSON, RJ
    SCHWARTZ, SE
    HALES, JM
    CESS, RD
    COAKLEY, JA
    HANSEN, JE
    HOFMANN, DJ
    [J]. SCIENCE, 1992, 255 (5043) : 423 - 430
  • [8] Substantial convection and precipitation enhancements by ultrafine aerosol particles
    Fan, Jiwen
    Rosenfeld, Daniel
    Zhang, Yuwei
    Giangrande, Scott E.
    Li, Zhanqing
    Machado, Luiz A. T.
    Martin, Scot T.
    Yang, Yan
    Wang, Jian
    Artaxo, Paulo
    Barbosa, Henrique M. J.
    Braga, Ramon C.
    Comstock, Jennifer M.
    Feng, Zhe
    Gao, Wenhua
    Gomes, Helber B.
    Mei, Fan
    Poehlker, Christopher
    Poehlker, Mira L.
    Poeschl, Ulrich
    de Souza, Rodrigo A. F.
    [J]. SCIENCE, 2018, 359 (6374) : 411 - +
  • [9] Potential aerosol indirect effects on atmospheric circulation and radiative forcing through deep convection
    Fan, Jiwen
    Rosenfeld, Daniel
    Ding, Yanni
    Leung, L. Ruby
    Li, Zhanqing
    [J]. GEOPHYSICAL RESEARCH LETTERS, 2012, 39
  • [10] Effects of aerosol optical properties on deep convective clouds and radiative forcing
    Fan, Jiwen
    Zhang, Renyi
    Tao, Wei-Kuo
    Mohr, Karen I.
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2008, 113 (D8)