Intrinsic magnetism in superconducting infinite-layer nickelates

被引:79
作者
Fowlie, Jennifer [1 ,2 ]
Hadjimichael, Marios [3 ]
Martins, Maria M. [4 ,5 ]
Li, Danfeng [1 ,6 ]
Osada, Motoki [1 ,7 ]
Wang, Bai Yang [1 ,8 ]
Lee, Kyuho [1 ,8 ]
Lee, Yonghun [1 ,2 ]
Salman, Zaher [4 ]
Prokscha, Thomas [4 ]
Triscone, Jean-Marc [3 ]
Hwang, Harold Y. [1 ,2 ]
Suter, Andreas [4 ]
机构
[1] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA
[2] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA
[3] Univ Geneva, Dept Quantum Matter Phys, Geneva, Switzerland
[4] Paul Scherrer Inst, Lab Muon Spin Spect, Villigen, Switzerland
[5] Swiss Fed Inst Technol, Adv Power Semicond Lab, Zurich, Switzerland
[6] City Univ Hong Kong, Dept Phys, Kowloon, Hong Kong, Peoples R China
[7] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA
[8] Stanford Univ, Dept Phys, Stanford, CA 94305 USA
基金
瑞士国家科学基金会; 欧洲研究理事会; 中国国家自然科学基金;
关键词
SPIN; EXCITATIONS;
D O I
10.1038/s41567-022-01684-y
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The discovery of superconductivity in Nd0.8Ar0.2NiO2 (ref. (1)) introduced a new family of layered nickelate superconductors that has now been extended to include a range of strontium doping(2,3), praseodymium or lanthanum in place of neodymium(4-7), and the five-layer compound Nd6Ni5O12 (ref. (8)). A number of studies have indicated that electron correlations are strong in these materials(9-15), a feature that often leads to the emergence of magnetism. Here we report muon spin rotation/relaxation studies of a series of superconducting infinite-layer nickelates. Regardless of the rare earth ion or doping, we observe an intrinsic magnetic ground state arising from local moments on the nickel sublattice. The coexistence of magnetism-which is likely to be antiferromagnetic and short-range ordered-with superconductivity is reminiscent of some iron pnictides(16) and heavy fermion compounds(17), and qualitatively distinct from the doped cuprates(18).
引用
收藏
页码:1043 / +
页数:6
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