Observations of atmospheric CO2 and CO based on in-situ and ground-based remote sensing measurements at Hefei site, China

被引：5

作者：

Shan, Changgong ^{[1
,8
]}

Wang, Wei ^{[1
]}

Xie, Yu ^{[6
]}

Wu, Peng ^{[1
]}

Xu, Jiaqing ^{[6
]}

Zeng, Xiangyu ^{[1
]}

Zha, Lingling ^{[6
]}

Zhu, Qianqian ^{[1
]}

Sun, Youwen ^{[1
]}

Hu, Qihou ^{[1
]}

Liu, Cheng ^{[1
,2
,3
,4
,5
]}

Jones, Nicholas ^{[7
]}

机构：

[1] Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Key Lab Environm Opt & Technol, Hefei 230031, Peoples R China

[2] Univ Sci & Technol China, Dept Precis Machinery & Precis Instrumentat, Hefei 230026, Peoples R China

[3] Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China

[4] Univ Sci & Technol China, Key Lab Precis Sci Instrumentat, Anhui Higher Educ Inst, Hefei 230026, Peoples R China

[5] Univ Sci & Technol China, Anhui Prov Key Lab Polar Environm & Global Change, Hefei 230026, Peoples R China

[6] Hefei Univ, Dept Automat, Hefei 230601, Anhui, Peoples R China

[7] Univ Wollongong, Sch Earth Atmospher & Life Sci, Northfields Ave, Wollongong, NSW 2522, Australia

[8] State Environm Protect Key Lab Sources & Control, Beijing 100084, Peoples R China

来源：

SCIENCE OF THE TOTAL ENVIRONMENT | 2022年 / 851卷

基金：

中国国家自然科学基金;

关键词：

CO2; CO; Remote sensing; Time-space distribution; Enhancement ratio of CO2 and CO; FOURIER-TRANSFORM SPECTROMETER; GASES OBSERVING SATELLITE; COLUMN-AVERAGED METHANE; LONG-TERM; CARBON-MONOXIDE; FTIR MEASUREMENTS; EASTERN CHINA; TIME-SERIES; EMISSIONS; TCCON;

D O I：

10.1016/j.scitotenv.2022.158188

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

The characteristics of long time series of CO2 and CO surface concentrations, tropospheric and total column dry-air mole fractions (DMF) from May 2015 to December 2019 were investigated. Both CO2 and CO show different seasonality for the three datasets. The annual increasing trend of CO2 is similar for all three datasets. However, the annual decreasing trend of CO for surface concentration is high compared to the other two measurements, mainly due to the improved combustion efficiency from power generation in recent years. The correlation between the tropospheric and total atmospheric CO2 and CO is higher than that between the surface concentration and tropospheric CO2 and CO. This is because the tropospheric and total atmospheric results both have common vertical profiles for CO2 and CO respective mole fractions that were observed in troposphere. Furthermore, the enhancement ratios of CO2 to CO derived from the three datasets during the period from 2016 to 2019 were compared. The ratio of delta CO2 to delta CO has an obvious increase with altitude each year, which means that the combustion efficiencies obtained from the three datasets are different. All ratios for the three datasets showed a slight increasing trend in recent years, which is attributed to increased combustion efficiency due to governmental measures for energy savings and emission reductions.

引用

页数：12

共 72 条

[1] Emission of trace gases and aerosols from biomass burning [J].

Andreae, MO ;

Merlet, P .

GLOBAL BIOGEOCHEMICAL CYCLES, 2001, 15 (04) :955-966

[2] Carbon monoxide (CO) and ethane (C2H6) trends from ground-based solar FTIR measurements at six European stations, comparison and sensitivity analysis with the EMEP model [J].

Angelbratt, J. ;

Mellqvist, J. ;

Simpson, D. ;

Jonson, J. E. ;

Blumenstock, T. ;

Borsdorff, T. ;

Duchatelet, P. ;

Forster, F. ;

Hase, F. ;

Mahieu, E. ;

De Maziere, M. ;

Notholt, J. ;

Petersen, A. K. ;

Raffalski, U. ;

Servais, C. ;

Sussmann, R. ;

Warneke, T. ;

Vigouroux, C. .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2011, 11 (17) :9253-9269

[3]

[Anonymous], 2014, [No title captured], P151

[4] Using XCO2 retrievals for assessing the long-term consistency of NDACC/FTIR data sets [J].

Barthlott, S. ;

Schneider, M. ;

Hase, F. ;

Wiegele, A. ;

Christner, E. ;

Gonzalez, Y. ;

Blumenstock, T. ;

Dohe, S. ;

Garcia, O. E. ;

Sepulveda, E. ;

Strong, K. ;

Mendonca, J. ;

Weaver, D. ;

Palm, M. ;

Deutscher, N. M. ;

Warneke, T. ;

Notholt, J. ;

Lejeune, B. ;

Mahieu, E. ;

Jones, N. ;

Griffith, D. W. T. ;

Velazco, V. A. ;

Smale, D. ;

Robinson, J. ;

Kivi, R. ;

Heikkinen, P. ;

Raffalski, U. .

ATMOSPHERIC MEASUREMENT TECHNIQUES, 2015, 8 (03) :1555-1573

[5]

Barthlott S., 2016, EARTH SYST SCI DATA, DOI [10.5194/essd-2016-9, DOI 10.5194/ESSD-2016-9]

[6] Multiannual changes of CO2 emissions in China: indirect estimates derived from satellite measurements of tropospheric NO2 columns [J].

Berezin, E. V. ;

Konovalov, I. B. ;

Ciais, P. ;

Richter, A. ;

Tao, S. ;

Janssens-Maenhout, G. ;

Beekmann, M. ;

Schulze, E. -D. .

ATMOSPHERIC CHEMISTRY AND PHYSICS, 2013, 13 (18) :9415-9438

[7] Source and meteorological influences on air quality (CO, CH4 & CO2) at a Southern Hemisphere urban site [J].

Buchholz, R. R. ;

Paton-Walsh, C. ;

Griffith, D. W. T. ;

Kubistin, D. ;

Caldow, C. ;

Fisher, J. A. ;

Deutscher, N. M. ;

Kettlewell, G. ;

Riggenbach, M. ;

Macatangay, R. ;

Krummel, P. B. ;

Langenfelds, R. L. .

ATMOSPHERIC ENVIRONMENT, 2016, 126 :274-289

[8] Retrieval of xCO2 from ground-based mid-infrared (NDACC) solar absorption spectra and comparison to TCCON [J].

Buschmann, Matthias ;

Deutscher, Nicholas M. ;

Sherlock, Vanessa ;

Palm, Mathias ;

Warneke, Thorsten ;

Notholt, Justus .

ATMOSPHERIC MEASUREMENT TECHNIQUES, 2016, 9 (02) :577-585

[9] Decreased Anthropogenic CO2 Emissions during the COVID-19 Pandemic Estimated from FTS and MAX-DOAS Measurements at Urban Beijing [J].

Cai, Zhaonan ;

Che, Ke ;

Liu, Yi ;

Yang, Dongxu ;

Liu, Cheng ;

Yue, Xu .

REMOTE SENSING, 2021, 13 (03) :1-12

[10] Contributions to accelerating atmospheric CO2 growth from economic activity, carbon intensity, and efficiency of natural sinks [J].

Canadell, Josep G. ;

Le Quéré, Corinne ;

Raupach, Michael R. ;

Field, Christopher B. ;

Buitenhuis, Erik T. ;

Ciais, Philippe ;

Conway, Thomas J. ;

Gillett, Nathan P. ;

Houghton, R. A. ;

Marland, Gregg .

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2007, 104 (47) :18866-18870

← 1 2 3 4 5 6 7 8 →