Tuning scalar spin chirality in ultrathin films of the kagome-lattice ferromagnet Fe3Sn

被引:6
作者
Fujiwara, Kohei [1 ]
Kato, Yasuyuki [2 ]
Seki, Takeshi [1 ,3 ]
Nomura, Kentaro [1 ,3 ]
Takanashi, Koki [1 ,3 ,4 ]
Motome, Yukitoshi [2 ]
Tsukazaki, Atsushi [1 ,3 ,4 ]
机构
[1] Tohoku Univ, Inst Mat Res, Sendai, Miyagi 9808577, Japan
[2] Univ Tokyo, Dept Appl Phys, Tokyo 1138656, Japan
[3] Tohoku Univ, Ctr Spintron Res Network CSRN, Sendai, Miyagi 9808577, Japan
[4] Tohoku Univ, Ctr Sci & Innovat Spintron CSIS, Core Res Cluster, Sendai, Miyagi 9808577, Japan
关键词
TEMPERATURE MAGNETIC SKYRMIONS; BERRY PHASE; DYNAMICS;
D O I
10.1038/s43246-021-00218-y
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Non-coplanar spin textures with finite scalar spin chirality can be artificially induced at surfaces and interfaces through the interfacial Dzyaloshinskii-Moriya interaction. However, stabilizing a proper magnetic skyrmion crystal via this route remains elusive. Here, using an epitaxial bilayer of platinum and geometrically frustrated kagome-lattice ferromagnet Fe3Sn, we show the possible formation of a two-dimensional skyrmion crystal under well-regulated Fe3Sn thickness conditions. Magnetization measurements reveal that the magnetic anisotropy is systematically varied from an inherent in-plane type to a perpendicular type with the thickness reduction. Below approximately 0.5 nm, we clearly detect a topological Hall effect that provides evidence for finite scalar spin chirality. Our topological Hall effect analysis, combined with theoretical simulations, not only establishes its interfacial Dzyaloshinskii-Moriya interaction origin, but also indicates the emergence of a stable skyrmion crystal phase, demonstrating the potential of kagome-lattice ferromagnets in spin chirality engineering using thin-film nanostructures. Magnetic skyrmions are swirling topological spin textures induced by chiral interactions in non-centrosymmetric systems. Here, a Pt-Fe3Sn bilayer exhibits a thickness-dependent magnetic anisotropy and interfacial Dzyaloshinskii-Moriya interaction that are key to the controlled stabilization of a skyrmion crystal.
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页数:7
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