A novel inorganic scintillator:: Lu2Si2O7:Ce3+ (LPS)

被引:86
作者
Pauwels, D
Le Masson, N
Viana, B
Kahn-Harari, A
van Loef, EVD
Dorenbos, P
van Eijk, CWE
机构
[1] ENSCP, Lab Chim Appl Etat Solide, CNRS, UMR 7574, F-75231 Paris 05, France
[2] Delft Univ Technol, Radiat Technol Grp, Interfac Reactor Inst, NL-2629 JB Delft, Netherlands
关键词
D O I
10.1109/23.914446
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
We have characterized the gamma and X-ray scintillation properties of Ce3+ doped Lu2Si2O7, a lutetium pyre-silicate (LPS) material. The rare earth ions are located in an octahedral site with C-2 symmetry. The compound exhibits chemical stability, transparency in a wide optical range and congruent melting, which allows growing of single crystals of good optical quality. The melting temperature is about 2000 degreesC, slightly lower than that of Lu2SiO5 (LSO). Two maxima at 305 nm and 355 nm are observed in the optical absorption spectrum. The emission spectrum of Ce3+ in LPS shows a broad band peaking at 380 nm. For a nominal Ce3+ atomic concentration of similar to0.01, under gamma-ray excitation we observe light yields in the range 13,000-23,000 photons/MeV, depending on the preparation atmosphere. The actual cerium concentration inside the crystal still needs to be determined. The scintillation decay time is around 30 ns and, in the first studies, neither a long component nor afterglow was observed.
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页码:1787 / 1790
页数:4
相关论文
共 11 条
[1]  
ANANEVA GV, 1982, IZVESTIYA AKAD NAUK, V3, P349
[2]  
BERTHEAURAYNAL F, 1981, J APPL CRYSTALLOGR, V14, P349
[3]  
Blasse G., Luminescent Materials
[4]   SYNTHESIS AND SPECTROSCOPIC STUDY OF LUTETIUM PYROSILICATE SINGLE-CRYSTALS DOPED WITH TRIVALENT EUROPIUM [J].
BRETHEAURAYNAL, F ;
TERCIER, N ;
BLANZAT, B ;
DRIFFORD, M .
MATERIALS RESEARCH BULLETIN, 1980, 15 (05) :639-646
[5]  
CHRISTENSEN AN, 1994, Z KRISTALLOGR, V209, P7
[6]  
Henderson B., 1989, OPTICAL SPECTROSCOPY
[7]  
MELCHER CL, 1998, NUCL INSTRUM METH B, V134, P304
[8]   Properties of the new LuAP:Ce scintillator [J].
Moszynski, M ;
Wolski, D ;
Ludziejewski, T ;
Kapusta, M ;
Lempicki, A ;
Brecher, C ;
Wisniewski, D ;
Wojtowicz, AJ .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1997, 385 (01) :123-131
[9]  
REVCOLEVSCHI A, 1968, CR ACAD SCI C CHIM, V266, P1767
[10]   REVISED EFFECTIVE IONIC-RADII AND SYSTEMATIC STUDIES OF INTERATOMIC DISTANCES IN HALIDES AND CHALCOGENIDES [J].
SHANNON, RD .
ACTA CRYSTALLOGRAPHICA SECTION A, 1976, 32 (SEP1) :751-767