Chemical pressure tuning of URu2Si2 via isoelectronic substitution of Ru with Fe

被引:33
作者
Das, Pinaki [1 ]
Kanchanavatee, N. [2 ,3 ]
Helton, J. S. [4 ,5 ]
Huang, K. [3 ,6 ]
Baumbach, R. E. [1 ,7 ]
Bauer, E. D. [1 ]
White, B. D. [2 ,3 ]
Burnett, V. W. [2 ,3 ]
Maple, M. B. [2 ,3 ,6 ]
Lynn, J. W. [5 ]
Janoschek, M. [1 ]
机构
[1] Los Alamos Natl Lab, MPA CMMS, Los Alamos, NM 87545 USA
[2] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA
[3] Univ Calif San Diego, Ctr Adv Nanosci, La Jolla, CA 92093 USA
[4] US Naval Acad, Dept Phys, Annapolis, MD 21402 USA
[5] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA
[6] Univ Calif San Diego, La Jolla, CA 92093 USA
[7] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA
基金
美国国家科学基金会;
关键词
HIDDEN-ORDER TRANSITION; FERMI-SURFACE; MAGNETIC EXCITATIONS; SYSTEM; SUPERCONDUCTIVITY; TEMPERATURE; RESISTIVITY; ENTROPY; LATTICE; MOMENT;
D O I
10.1103/PhysRevB.91.085122
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have used specific heat and neutron diffraction measurements on single crystals of URu2-xFexSi2 for Fe concentrations x <= 0.7 to establish that chemical substitution of Ru with Fe acts as "chemical pressure" P-ch as previously proposed by Kanchanavatee et al. [Phys. Rev. B 84, 245122 ( 2011)] based on bulk measurements on polycrystalline samples. Notably, neutron diffraction reveals a sharp increase of the uranium magnetic moment at x = 0.1, reminiscent of the behavior at the "hidden order" to large-moment-antiferromagnetic phase transition observed at a pressure Px approximate to 0.5-0.7 GP(a) in URu2Si2. Using the unit-cell volume determined from our measurements and an isothermal compressibility kappa(T) = 5.2 x 10(-3) GPa(-1) for URu2Si2, we determine the chemical pressure Pch in URu2-xFexSi2 as a function of x. The resulting temperature (T)-chemical pressure ( P-ch) phase diagram for URu2-xFexSi2 is in agreement with the established temperature (T)-external pressure (P) phase diagram of URu2Si2.
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页数:6
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