Self-assembled three-dimensional chiral colloidal architecture

被引：111
作者：
Ben Zion, Matan Yah [1 ]
He, Xiaojin [1 ]
Maass, Corinna C. [1 ,2 ]
Sha, Ruojie [3 ]
Seeman, Nadrian C. [3 ]
Chaikin, Paul M. [1 ]
机构：
[1] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA
[2] Max Planck Inst Dynam & Self Org, Fassberg 17, D-37077 Gottingen, Germany
[3] NYU, Dept Chem, New York, NY 10003 USA
来源：
SCIENCE | 2017年 / 358卷 / 6363期
关键词：
DNA; PATTERNS;
D O I：
10.1126/science.aan5404
中图分类号：
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号：
07 ; 0710 ; 09 ;
摘要：
Although stereochemistry has been a central focus of the molecular sciences since Pasteur, its province has previously been restricted to the nanometric scale. We have programmed the self-assembly of micron-sized colloidal clusters with structural information stemming from a nanometric arrangement. This was done by combining DNA nanotechnology with colloidal science. Using the functional flexibility of DNA origami in conjunction with the structural rigidity of colloidal particles, we demonstrate the parallel self-assembly of three-dimensional microconstructs, evincing highly specific geometry that includes control over position, dihedral angles, and cluster chirality.
引用
收藏
页码：633 / +
页数：4
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