Temperature induced high charge-discharge performances in lead-free Bi0.5Na0.5TiO3-based ergodic relaxor ferroelectric ceramics

被引:165
作者
Li, Feng [1 ,2 ,3 ]
Yang, Ke [1 ]
Liu, Xing [1 ]
Zou, Jian [2 ,3 ]
Zhai, Jiwei [1 ]
Shen, Bo [1 ]
Li, Peng [1 ]
Shen, Jie [1 ]
Liu, Baihui [1 ]
Chen, Pan [1 ]
Zhao, Kunyu [2 ]
Zeng, Huarong [2 ]
机构
[1] Tongji Univ, Sch Mat Sci & Engn, Key Lab Adv Civil Engn Mat, Minist Educ, 4800 Caoan Rd, Shanghai 201804, Peoples R China
[2] Chinese Acad Sci, Shanghai Inst Ceram, key Lab Inorgan Funct Mat & Devices, Shanghai 200050, Peoples R China
[3] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
基金
国家重点研发计划;
关键词
BNT-based; Lead-free ceramic; Charge-discharge; Energy storage; ENERGY-STORAGE PROPERTIES; ANTIFERROELECTRIC CERAMICS; PHASE-TRANSITION; ELECTROSTRICTIVE STRAIN; FREE PIEZOCERAMICS; SOLID-SOLUTIONS; FIELD; DIELECTRICS; CAPACITORS; DEPENDENCE;
D O I
10.1016/j.scriptamat.2017.07.010
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The temperature dependence of energy storage and charge-discharge properties of a lead-free 0.62Bi(0.5)Na(0.5)TiO(3)-0.06BaTiO(3)-0.32(Sr0.7Bi0.2 square(0.1))TiO3 ergodic relaxor ferroelectric ceramic were investigated. The energy storage density was maintained >= 0.5 J/cm(3) up to 140 degrees C with a high efficiency >= 90%. The stored energy was released in sub-microsecond durations and charge-discharge performances were enhanced as temperature increased to 160 degrees C. This ceramic possessed an enhanced power density 182 MW/cm(3) and large current density 606 A/cm(2). All results showed that this ergodic relaxor ferroelectric ceramics appeared very promising for pulse capacitor applications. (C) 2017 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:15 / 19
页数:5
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