Recent progress of electrocatalysts for oxygen reduction in fuel cells

被引：120

作者：

Liu, Mingyang ^{[1
,2
]}

Xiao, Xudong ^{[1
]}

Li, Qi ^{[1
]}

Luo, Laiyu ^{[1
]}

Ding, Minghui ^{[2
]}

Zhang, Bin ^{[2
,3
]}

Li, Yuxin ^{[1
]}

Zou, Jinlong ^{[1
]}

Jiang, Baojiang ^{[1
]}

机构：

[1] Heilongjiang Univ, Sch Chem & Mat Sci, Key Lab Funct Inorgan Mat Chem, Minist Educ Peoples Republ China, Harbin 150080, Peoples R China

[2] Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin, Heilongjiang, Peoples R China

[3] Heilongjiang Acad Sci, Inst Petr Chem, Harbin, Heilongjiang, Peoples R China

来源：

JOURNAL OF COLLOID AND INTERFACE SCIENCE | 2022年 / 607卷

基金：

中国国家自然科学基金;

关键词：

Electrocatalysis; Oxygen reduction reaction; Platinum group metal; Transition metal compounds; Carbon-based electrocatalysts; N-DOPED CARBON; METAL-ORGANIC FRAMEWORKS; POROUS CARBON; EFFICIENT CATALYSTS; BIFUNCTIONAL ELECTROCATALYST; HYDROGEN EVOLUTION; MESOPOROUS CARBON; ALKALINE MEDIA; ORR ACTIVITY; NITROGEN;

D O I：

10.1016/j.jcis.2021.09.008

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Oxygen reduction reaction (ORR) has gradually been in the limelight in recent years because of its great application potential for fuel cells and rechargeable metal-air batteries. Therefore, significant issues are increasingly focused on developing effective and economical ORR electrocatalysts. This review begins with the reaction mechanisms and theoretical calculations of ORR in acidic and alkaline media. The latest reports and challenges in ORR electrocatalysis are traced. Most importantly, the latest advances in the development of ORR electrocatalysts are presented in detail, including platinum group metal (PGM), transition metal, and carbon-based electrocatalysts with various nanostructures. Furthermore, the development prospects and challenges of ORR electrocatalysts are speculated and discussed. These insights would help to formulate the design guidelines for highly-active ORR electrocatalysts and affect future research to obtain new knowledge for ORR mechanisms. (c) 2021 Elsevier Inc. All rights reserved.

引用

页码：791 / 815

页数：25

共 199 条

[41] Tailoring the nano heterointerface of hematite/magnetite on hierarchical nitrogen-doped carbon nanocages for superb oxygen reduction [J].