Ultrahigh Thermoelectric Performance in Mosaic Crystals

被引:221
作者
He, Ying [1 ,2 ,3 ]
Lu, Ping [1 ,3 ]
Shi, Xun [1 ,2 ]
Xu, Fangfang [1 ]
Zhang, Tiansong [2 ]
Snyder, Gerald Jeffrey [4 ]
Uher, Ctirad [5 ]
Chen, Lidong [1 ,2 ,6 ]
机构
[1] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China
[2] Chinese Acad Sci, Shanghai Inst Ceram, CAS Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China
[3] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[4] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA
[5] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA
[6] Shanghai Inst Mat Genome, Shanghai 200444, Peoples R China
基金
中国国家自然科学基金;
关键词
FIGURE; SCATTERING; HEAT;
D O I
10.1002/adma.201501030
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Successful research strategies to enhance the dimensionless figure of merit zT above 2 rely on either bulk nanomaterials or on single crystals. A new physical mechanism of nanoscale mosaicity is shown that goes beyond the approaches in single crystals or conventional nanomaterials. A zT value of 2.1 at 1000 K in bulk nanomaterials is achieved.
引用
收藏
页码:3639 / 3644
页数:6
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