Emerging trends in porous materials for CO2capture and conversion

被引:589
作者
Singh, Gurwinder [1 ]
Lee, Jangmee [1 ]
Karakoti, Ajay [1 ]
Bahadur, Rohan [1 ]
Yi, Jiabao [1 ]
Zhao, Dongyuan [2 ]
AlBahily, Khalid [3 ]
Vinu, Ajayan [1 ]
机构
[1] Univ Newcastle, Global Innovat Ctr Adv Nanomat, Fac Engn & Built Environm, Callaghan, NSW 2308, Australia
[2] Fudan Univ, Dept Chem, Lab Adv Nanomat, IChEM Collaborat Innovat Ctr Chem Energy Mat, Shanghai 200433, Peoples R China
[3] KAUST, SABIC Corp Res & Dev Ctr, Saudi Basic Ind Corp, Thuwal 23955, Saudi Arabia
基金
澳大利亚研究理事会;
关键词
METAL-ORGANIC FRAMEWORK; CARBON-DIOXIDE CAPTURE; CONJUGATED MICROPOROUS POLYMERS; HIGH-SURFACE-AREA; EFFICIENT CO2 ADSORPTION; ORDERED MESOPOROUS CARBON; CROSS-LINKED POLYMERS; LEWIS BASIC SITES; COAL-TAR PITCH; ACTIVATED CARBON;
D O I
10.1039/d0cs00075b
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The presence of an excessive concentration of CO(2)in the atmosphere needs to be curbed with suitable measures including the reduction of CO(2)emissions at stationary point sources such as power plants through carbon capture technologies and subsequent conversion of the captured CO(2)into non-polluting clean fuels/chemicals using photo and/or electrocatalytic pathways. Porous materials have attracted much attention for carbon capture and in the recent past; they have witnessed significant advancements in their design and implementation for CO(2)capture and conversion. In this context, the emerging trends in major porous adsorbents such as MOFs, zeolites, POPs, porous carbons, and mesoporous materials for CO(2)capture and conversion are discussed. Their surface texture and chemistry, and the influence of various other features on their efficiency, selectivity, and recyclability for CO(2)capture and conversion are explained and compared thoroughly. The scientific and technical advances on the material structureversusCO(2)capture and conversion provide deep insights into designing effective porous materials. The review concludes with a summary, which compiles the key challenges in the field, current trends and critical challenges in the development of porous materials, and future research directions combined with possible solutions for realising the deployment of porous materials in CO(2)capture and conversion.
引用
收藏
页码:4360 / 4404
页数:45
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