Terahertz radiation and second-harmonic generation from InAs: Bulk versus surface electric-field-induced contributions

被引:98
作者
Reid, M [1 ]
Cravetchi, IV [1 ]
Fedosejevs, R [1 ]
机构
[1] Univ Alberta, Dept Elect & Comp Engn, Edmonton, AB T6G 2V4, Canada
关键词
D O I
10.1103/PhysRevB.72.035201
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Polarized second-harmonic generation and terahertz radiation in reflection from (100), (110), and (111) faces of n-type InAs crystals are investigated as a function of the sample azimuthal orientation under excitation from femtosecond Ti:sapphire laser pulses. The expressions describing the second-order response (optical second-harmonic generation and optical rectification) in reflection from zinc-blende crystals, such as InAs, are calculated taking into account the bulk electric-dipole contribution and the first-order surface electric-field-induced contribution. It is shown that the two contributions can be separated based on rotation symmetry considerations. Moreover, a direct comparison of the second-harmonic generation and terahertz radiation emission indicates that the observed dominant surface electric-field-induced optical rectification component may be attributed to the large free-carrier contribution to the third-order susceptibility in InAs.
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页数:9
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共 40 条
[1]  
Adachi S., 1999, Optical Constants of Crystalline and Amorphous Semiconductors Numerical Data and Graphical Information, V1st ed.
[2]   Terahertz emission from p-InAs due to the instantaneous polarization [J].
Adomavicius, R ;
Urbanowicz, A ;
Molis, G ;
Krotkus, A ;
Satkovskis, E .
APPLIED PHYSICS LETTERS, 2004, 85 (13) :2463-2465
[3]   PICOSECOND PHOTOCONDUCTING HERTZIAN DIPOLES [J].
AUSTON, DH ;
CHEUNG, KP ;
SMITH, PR .
APPLIED PHYSICS LETTERS, 1984, 45 (03) :284-286
[4]   Surface nonlinear optics: a historical overview [J].
Bloembergen, N .
APPLIED PHYSICS B-LASERS AND OPTICS, 1999, 68 (03) :289-293
[5]  
Boyd R. W., 2003, NONLINEAR OPTICS
[6]   RAMAN-SCATTERING AT (111) AND (111) SURFACES OF N-INAS AND P-INAS [J].
BUCHNER, S ;
CHING, LY ;
BURSTEIN, E .
PHYSICAL REVIEW B, 1976, 14 (10) :4459-4462
[7]  
Butcher PN., 1990, Cambridge Studies in Modern Optics, DOI 10.1017/CBO9781139167994
[8]   CALCULATION OF OPTICAL-EXCITATIONS IN CUBIC SEMICONDUCTORS .3. 3RD-HARMONIC GENERATION [J].
CHING, WY ;
HUANG, MZ .
PHYSICAL REVIEW B, 1993, 47 (15) :9479-9491
[9]   OPTICAL RECTIFICATION AT SEMICONDUCTOR SURFACES [J].
CHUANG, SL ;
SCHMITTRINK, S ;
GREENE, BI ;
SAETA, PN ;
LEVI, AFJ .
PHYSICAL REVIEW LETTERS, 1992, 68 (01) :102-105
[10]   THz electromagnetic emission by coherent infrared-active phonons [J].
Dekorsy, T ;
Auer, H ;
Bakker, HJ ;
Roskos, HG ;
Kurz, H .
PHYSICAL REVIEW B, 1996, 53 (07) :4005-4014