Collective escape processes in many-particle systems

被引:2
作者
Fugmann, S. [1 ]
Hennig, D. [2 ]
Schimansky-Geier, L. [1 ]
Sokolov, I. M. [1 ]
机构
[1] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany
[2] Univ Portsmouth, Dept Math, Portsmouth PO1 3HF, Hants, England
关键词
CONTROLLED INTRACHAIN REACTIONS; ENERGY LOCALIZATION; POLYMERS; CHAIN;
D O I
10.1140/epjst/e2010-01350-8
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We study collective escape phenomena in nonlinear chain models. First we investigate the fragmentation of an overdamped polymer chain due to thermal fluctuations in the absence of an external force. We calculate the activation times of individual bonds in the coupled chain system and compare them with times obtained from Brownian dynamics simulations. We also consider a grafted chain exposed to an external force which monotonically grows as time goes on. In underdamped situations we show that collective localized excitations in a nonlinear force field with absorbing states can cause polymer fragmentation. In a similar fashion, localized modes assist a thermally activated escape of interacting particles in a metastable potential landscape which is additionally subjected to a periodic driving. The latter is necessary to obtain overcritical elongations which create localized modes even in case of stronger damping.
引用
收藏
页码:187 / 210
页数:24
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