The Influence of Ce or Mn Doping on Cu-Based Catalysts for De-NOx with NH3-SCR

被引:18
作者
Jiang, Lei [1 ]
Ca, Yixi [1 ]
Jin, Miaomiao [1 ]
Zhu, Zengzan [2 ]
Wang, Yinhuan [2 ]
机构
[1] Jiangsu Univ, Sch Automot & Transportat Engn, Zhenjiang 212013, Jiangsu, Peoples R China
[2] Kailong Lanfeng New Mat Technol Co Ltd, Zhenjiang 212132, Jiangsu, Peoples R China
关键词
CU-SAPO-34; CATALYSTS; REDUCTION; PERFORMANCE; STABILITY; AMMONIA; NH3; SCR; CU-SSZ-13;
D O I
10.1155/2020/1462801
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this study, the de-NOx performance of Cu-based zeolite catalysts supported on topological structure (SSZ-13, BEA, ZSM-5) and loaded with different doses of copper (from 2 to 6 wt.%) was investigated. The preparation of copper-based catalysts adopted the incipient wetness impregnation method. To analyze the physicochemical properties of the catalysts, advanced techniques like BET, XRD, NH3-TPD, H-2-TPR, and DRS UV-Vis were used. The performance tests suggested the 4Cu/SSZ-13 catalyst exhibited higher low-temperature activity and wider temperature window. Furthermore, compared with Mn-Cu/SSZ-13, the Ce-Cu/SSZ-13 catalysts exhibited better de-NOx performance.
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页数:8
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