Dynamics of active liquid interfaces

被引:65
作者
Adkins, Raymond [1 ]
Kolvin, Itamar [1 ]
You, Zhihong [1 ]
Witthaus, Sven [1 ]
Marchetti, M. Cristina [1 ,2 ]
Dogic, Zvonimir [1 ,2 ]
机构
[1] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA
[2] Univ Calif Santa Barbara, Grad Program Biomol Sci & Engn, Santa Barbara, CA 93106 USA
关键词
D O I
10.1126/science.abo5423
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Controlling interfaces of phase-separating fluid mixtures is key to the creation of diverse functional soft materials. Traditionally, this is accomplished with surface-modifying chemical agents. Using experiment and theory, we studied how mechanical activity shapes soft interfaces that separate an active and a passive fluid. Chaotic flows in the active fluid give rise to giant interfacial fluctuations and noninertial propagating active waves. At high activities, stresses disrupt interface continuity and drive droplet generation, producing an emulsion-like active state composed of finite-sized droplets. When in contact with a solid boundary, active interfaces exhibit nonequilibrium wetting transitions, in which the fluid climbs the wall against gravity. These results demonstrate the promise of mechanically driven interfaces for creating a new class of soft active matter.
引用
收藏
页码:768 / 772
页数:5
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