Water at Interfaces

被引：578

作者：

Bjornehohn, E. ^{[1
]}

Hansen, Martin H. ^{[2
,8
]}

Hodgson, Andrew ^{[3
]}

Liu, Li-Min ^{[4
,5
,6
]}

Limmer, David T. ^{[7
]}

Michaelides, Angelos ^{[4
,5
]}

Pedevilla, Philipp ^{[4
,5
]}

Rossmeisl, Jan ^{[8
]}

Shen, Huaze ^{[9
,10
]}

Tocci, Gabriele ^{[4
,5
,14
,15
]}

Tyrode, Eric ^{[11
]}

Walz, Marie-Madeleine ^{[1
,16
]}

Werner, Josephina ^{[1
,12
]}

Bluhm, Hendrik ^{[13
]}

机构：

[1] Uppsala Univ, Dept Phys & Astron, BOX 516, S-75120 Uppsala, Sweden

[2] Tech Univ Denmark, DK-2800 Lyngby, Denmark

[3] Univ Liverpool, Dept Chem, Liverpool L69 7ZD, Merseyside, England

[4] UCL, London Ctr Nanotechnol, Thomas Young Ctr, Dept Phys & Astron, London WC1E 6BT, England

[5] UCL, Dept Chem, London WC1E 6BT, England

[6] Beijing Computat Sci Res Ctr, Beijing 100193, Peoples R China

[7] Princeton Univ, Princeton Ctr Theoret Sci, Princeton, NJ 08544 USA

[8] Univ Copenhagen, Dept Chem, Univ Pk 5, DK-2100 Copenhagen, Denmark

[9] Peking Univ, Int Ctr Quantum Mat, Beijing 100871, Peoples R China

[10] Peking Univ, Sch Phys, Beijing 100871, Peoples R China

[11] KTH Royal Inst Technol, Dept Chem, S-10044 Stockholm, Sweden

[12] Swedish Univ Agr Sci, Dept Chem & Biotechnol, Box 7015, S-75007 Uppsala, Sweden

[13] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA

[14] Ecole Polytech Fed Lausanne, Sch Engn, Inst Bioengn & Mat Sci & Engn, Lab Fundamental BioPhoton,Lab Computat Sci & Mode, CH-1015 Lausanne, Switzerland

[15] Ecole Polytech Fed Lausanne, Lausanne Ctr Ultrafast Sci, CH-1015 Lausanne, Switzerland

[16] Uppsala Univ, Dept Cell & Mol Biol, Box 596, SE-75124 Uppsala, Sweden

来源：

CHEMICAL REVIEWS | 2016年 / 116卷 / 13期

基金：

瑞典研究理事会; 欧洲研究理事会;

关键词：

DENSITY-FUNCTIONAL THEORY; SUM-FREQUENCY SPECTROSCOPY; MOLECULAR-DYNAMICS SIMULATIONS; SITU X-RAY; LIQUID-VAPOR INTERFACE; PHOTOELECTRON-SPECTROSCOPY; HYDROPHOBIC SURFACES; AQUEOUS-SOLUTION; ELECTROCHEMICAL INTERFACE; COMPUTER-SIMULATIONS;

D O I：

10.1021/acs.chemrev.6b00045

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The interfaces of neat water and aqueous solutions play a prominent role in many technological processes and in the environment. Examples of aqueous interfaces are ultrathin water films that cover most hydrophilic surfaces under ambient relative humidities, the liquid/solid interface which drives many electrochemical reactions, and the liquid/vapor interface, which governs the uptake and release of trace gases by the oceans and cloud droplets. In this article we review some of the recent experimental and theoretical advances in our knowledge of the properties of aqueous interfaces and discuss open questions and gaps in our understanding.

引用

页码：7698 / 7726

页数：29

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