Optimized design of an electrochemical filter-press reactor using CFD methods

被引:45
作者
Frias-Ferrer, Angel [1 ,2 ]
Tudela, Ignacio [1 ,2 ]
Louisnard, Olivier [3 ]
Saez, Veronica [1 ,2 ]
Deseada Esclapez, Maria [2 ,4 ]
Isabel Diez-Garcia, Maria [1 ,2 ]
Bonete, Pedro [2 ,4 ]
Gonzalez-Garcia, Jose [1 ,2 ]
机构
[1] Univ Alicante, Dept Quim Fis, Grp Nuevos Desarrollos Tecnol Electroquim Sonoele, E-03080 Alicante, Spain
[2] Univ Alicante, Inst Univ Electroquim, E-03080 Alicante, Spain
[3] Univ Toulouse, Ecole Mines Albi, Ctr RAPSODEE, FRE CNRS 3213, F-81013 Albi, France
[4] Univ Alicante, Dept Quim Fis, Grp Fotoquim & Electroquim Semicond, E-03080 Alicante, Spain
关键词
CFD; Electrochemistry; Filter-press reactor; Hydrodynamics; Laminar flow; Mass transfer; RTD; RESIDENCE TIME DISTRIBUTION; MASS-TRANSFER; HYDRODYNAMIC BEHAVIOR; FLOW VISUALIZATION; WASTE-WATER; ELECTRODE; TRANSPORT; VIABILITY; COPPER; CELL;
D O I
10.1016/j.cej.2011.02.053
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A former laboratory filter-press electrochemical reactor previously used in electrodialysis,electrosynthesis and wastewater treatment was studied from a hydrodynamic point of view using computational fluid dynamics (CFD). A finite elements method (FEM) software environment was used in order to simulate both fluid velocity field and tracer diffusion in the reactor for different low Reynolds numbers, enabling the estimation of active and stagnant areas inside the reactor. These results provided interesting information in order to design a new electrochemical compartment focusing on the entrance-exit manifolds to minimize the formation of stagnant areas within the reactor. CFD methods were again employed to study and optimize the new reactor in order to predict its performance. In both cases, CFD calculations were compared with residence time distribution (RID) studies in order to validate the simulations. (C) 2011 Elsevier B.V. All rights reserved.
引用
收藏
页码:270 / 281
页数:12
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