Chlorobismuthates Trapping Dibromine: Formation of Two-Dimensional Supramolecular Polyhalide Networks with Br2 Linkers

被引：50
|
作者：
Adonin, Sergey A. [1 ,2 ]
Gorokh, Igor D. [2 ]
Abramov, Pavel A. [1 ,2 ]
Novikov, Alexander S. [3 ]
Korolkov, Ilya V. [1 ,2 ]
Sokolov, Maxim N. [1 ,2 ]
Fedin, Vladimir P. [1 ,2 ]
机构：
[1] Russian Acad Sci, Nikolaev Inst Inorgan Chem SB, Lavrentieva St 3, Novosibirsk 630090, Russia
[2] Novosibirsk State Univ, Pirogova St 2, Novosibirsk 630090, Russia
[3] St Petersburg State Univ, Inst Chem, Univ Skaya Nab 7-9, St Petersburg 199034, Russia
来源：
EUROPEAN JOURNAL OF INORGANIC CHEMISTRY | 2017年 / 42期
基金：
俄罗斯科学基金会; 俄罗斯基础研究基金会;
关键词：
Polyhalides; Halogens; QTAIM; Density functional calculations; Halometalates; CRYSTAL-STRUCTURE; IONIC-LIQUID; COMPLEXES; BROMINE; HALOGEN; ANIONS; NONABROMOANTIMONATE(V); TRIBROMIDE; CHEMISTRY; COMPOUND;
D O I：
10.1002/ejic.201700908
中图分类号：
O61 [无机化学];
学科分类号：
070301 ; 081704 ;
摘要：
Reactions between BiCl3, Br-2, and chlorides of pyridinium (1), 4,4-propylenedipyridinium (2), or trimethylphenylammonium (3) in aqueous HCl lead to the formation of chlorobismuthate complexes trapping {Br-2} in the solid state into two-dimensional polyhalide supramolecular networks. The nature of non-covalent Br<bold>Cl interactions was studied by theoretical methods</bold>; estimated energies of these interactions are 1.9-6.0 kcal/mol.
引用
收藏
页码：4925 / 4929
页数：5
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