Accelerated Discovery of Thermoelectric Materials: Combinatorial Facility and High-Throughput Measurement of Thermoelectric Power Factor

被引:14
作者
Garcia-Canadas, Jorge [1 ,4 ]
Adkins, Nicholas J. E. [2 ]
McCain, Stephen [2 ]
Hauptstein, Bastian [2 ]
Brew, Ashley [1 ]
Jarvis, David J. [3 ]
Min, Gao [1 ]
机构
[1] Cardiff Univ, Sch Engn, Cardiff CF24 3AA, S Glam, Wales
[2] Univ Birmingham, Coll Engn & Phys Sci, Birmingham B15 2TT, W Midlands, England
[3] European Space Agcy, Keplerlaan 1,POB 299, NL-2200 AG Noordwijk, Netherlands
[4] Univ Jaume 1, Dept Ind Syst Engn & Design, Campus Riu Sec, Castellon de La Plana 12071, Spain
关键词
high-throughput; thermoelectric materials; laser processing; combinatorial chemistry; power factor; FE;
D O I
10.1021/acscombsci.5b00178
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
A series of processes have been developed to facilitate the rapid discovery of new promising thermoelectric alloys. A novel combinatorial facility where elements are wire fed and laser-melted was designed and constructed. Different sample compositions can be achieved by feeding different element wires at specific rates. The composition of all the samples prepared was tested by energy dispersive X-ray spectroscopy (EDS). Then, their thermoelectric properties (power factor) at room temperature were screened in a specially designed new high-throughput setup. After the screening, the thermoelectric properties can be mapped with the possibility of identifying compositional trends. As a promising thermoelectric ternary system, Al-Fe-Ti, has been identified, demonstrating the capability approach.
引用
收藏
页码:314 / 319
页数:6
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