The effect of pulsating pressure on the performance of a PEM fuel cell with a wavy cathode surface

被引:50
作者
Ashorynejad, Hamid Reza [1 ]
Javaherdeh, Koroush [1 ]
Van den Akker, Harry E. A. [2 ]
机构
[1] Univ Guilan, Dept Mech Engn, Rasht, Iran
[2] Delft Univ Technol, Dept Chem Engn, Fac Sci Appl, NL-2600 AA Delft, Netherlands
关键词
PEM fuel cell; Pressure pulsation; Wavy wall; Pore-scale modeling; Heterogeneous GDL; Lattice Boltzmann method; LATTICE BOLTZMANN METHOD; MASS-TRANSFER ENHANCEMENT; LIQUID WATER TRANSPORT; GAS-DIFFUSION LAYER; NUMERICAL-SIMULATION; GRID REFINEMENT; FLOW CHANNEL; ELECTRODE; MODEL; PERMEABILITY;
D O I
10.1016/j.ijhydene.2016.05.291
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In the context of attempts to improve the performance of Proton Exchange Membrane (PEM) fuel cells with a heterogeneous porous gas diffusion layer (GDL) consisting of carbon paper, we investigated whether - and to which degree - pulsating the pressure in a single waveform cathode channel affects the flow field in the channel and the performance of the fuel cell. In this 2-D study, the GDL was modeled by a stochastic arrangement of circular solid obstacles the macroscopic transport properties of which, such as permeability and tortuosity, were numerically simulated and found to compare favorably with experimental data. The focus of this paper is on the effects of varying amplitude and frequency of the pressure pulsations on cell performance. The results obtained show that a pulsating pressure "enhances the convective species transport to the reaction sites and thereby increases cell performance. We found that in a waveform channel a pulsatile pressure with an amplitude as high as 0.7 times the pressure drop over the cathode channel improves the fuel cell performance by around 7%, while the effect of pulsation frequency on output power is marginally small only. (C) 2016 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:14239 / 14251
页数:13
相关论文
共 50 条
[21]   Finite-Difference Lattice-BGK methods on nested grids [J].
Kandhai, D ;
Soll, W ;
Chen, S ;
Hoekstra, A ;
Sloot, P .
COMPUTER PHYSICS COMMUNICATIONS, 2000, 129 (1-3) :100-109
[22]   Lattice Boltzmann Method for Reacting Flows in Porous Media [J].
Kang, Qinjun ;
Lichtner, Peter C. ;
Janecky, David R. .
ADVANCES IN APPLIED MATHEMATICS AND MECHANICS, 2010, 2 (05) :545-563
[23]   Developing a new form of the Kozeny-Carman parameter for structured porous media through lattice-Boltzmann modeling [J].
Khabbazi, A. Ebrahimi ;
Ellis, J. S. ;
Bazylak, A. .
COMPUTERS & FLUIDS, 2013, 75 :35-41
[24]   Lattice Boltzmann simulation of liquid water transport in microporous and gas diffusion layers of polymer electrolyte membrane fuel cells [J].
Kim, Kwang Nam ;
Kang, Jung Ho ;
Lee, Sang Gun ;
Nam, Jin Hyun ;
Kim, Charn-Jung .
JOURNAL OF POWER SOURCES, 2015, 278 :703-717
[25]   Permeability and effective porosity of porous media [J].
Koponen, A ;
Kataja, M ;
Timonen, J .
PHYSICAL REVIEW E, 1997, 56 (03) :3319-3325
[26]   Evaluating the enhanced performance of a novel wave-like form gas flow channel in the PEMFC using the field synergy principle [J].
Kuo, Jenn-Kun ;
Chen, Cha'o-Kuang .
JOURNAL OF POWER SOURCES, 2006, 162 (02) :1122-1129
[27]   Three-dimensional numerical analysis of PEM fuel cells with straight and wave-like gas flow fields channels [J].
Kuo, Jenn-Kun ;
Yen, Tzu-Hsiang ;
Chen, Cha'o-Kuang .
JOURNAL OF POWER SOURCES, 2008, 177 (01) :96-103
[28]   The effects of buoyancy on the performance of a PEM fuel cell with a wave-like gas flow channel design by numerical investigation [J].
Kuo, Jenn-Kun ;
Chen, Cha'o-Kuang .
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 2007, 50 (21-22) :4166-4179
[29]   Three-dimensional transport model of PEM fuel cell with straight flow channels [J].
Liu, Xunliang ;
Tao, Wenquan ;
Li, Zengyao ;
He, Yaling .
JOURNAL OF POWER SOURCES, 2006, 158 (01) :25-35
[30]   Development and application of a generalised steady-state electrochemical model for a PEM fuel cell [J].
Mann, RF ;
Amphlett, JC ;
Hooper, MAI ;
Jensen, HM ;
Peppley, BA ;
Roberge, PR .
JOURNAL OF POWER SOURCES, 2000, 86 (1-2) :173-180