[1] British Geol Survey, Edinburgh EH9 3LA, Midlothian, Scotland
[2] British Geol Survey, Nottingham NG12 5GG, England
[3] NERC Isotope Geosci Labs, Nottingham NG12 5GG, England
[4] Cardiff Univ, Sch Earth & Ocean Sci, Cardiff CF10 3YE, S Glam, Wales