Design Improvement of Immobilized Photocatalytic Reactors Using a CFD-Taguchi Combined Method

被引:19
作者
Duran, J. Esteban [1 ]
Mohseni, Madjid [1 ]
Taghipour, Fariborz [1 ]
机构
[1] Univ British Columbia, Dept Chem & Biol Engn, Vancouver, BC V6T 1Z3, Canada
关键词
2,4-DICHLOROPHENOXYACETIC ACID; HEAT-TRANSFER; OPTIMIZATION; SURFACE; WATER; PHARMACEUTICALS; SIMULATION; MODEL; FIELD;
D O I
10.1021/ie101736d
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
An effective optimization design approach which combines CFD modeling and the Taguchi DOE method is presented for immobilized photocatalytic annular reactors used for water treatment. The analyzed reactor design incorporated the use of repeated ribs for improving the external mass transfer to the TiO2-coated wall. The CFD model was experimentally evaluated using 2,4-D as a model pollutant, providing close predictions of the photocatalytic degradation performance of the photoreactors over a wide range of Reynolds numbers (300 < Re < 10 000). The statistical analysis showed that the performance of the studied annular photocatalytic reactors was improved up to 60% using the ribs. A comparison of different reactor design factors indicated that better performance can be obtained using small outer tube diameters, large inner/outer tube diameter ratios, large (rib height)/(hydraulic diameter) ratio, and small (rib pitch)/(rib height) ratios. In addition, it was concluded that the (rib height)/(hydraulic diameter) ratio was the design parameter having the greatest impact (57%) on photoreactor performance.
引用
收藏
页码:824 / 831
页数:8
相关论文
共 36 条
[1]   A NEW TURBULENCE MODEL FOR PREDICTING FLUID-FLOW AND HEAT-TRANSFER IN SEPARATING AND REATTACHING FLOWS .1. FLOW-FIELD CALCULATIONS [J].
ABE, K ;
KONDOH, T ;
NAGANO, Y .
INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 1994, 37 (01) :139-151
[2]   Industrial exploitation of photocatalysis: progress, perspectives and prospects [J].
Adesina, AA .
CATALYSIS SURVEYS FROM ASIA, 2004, 8 (04) :265-273
[3]   Pharmaceuticals and personal care products (PPCPs) in surface and treated waters of Louisiana, USA and Ontario, Canada [J].
Boyd, GR ;
Reemtsma, H ;
Grimm, DA ;
Mitra, S .
SCIENCE OF THE TOTAL ENVIRONMENT, 2003, 311 (1-3) :135-149
[4]   Study and optimization of an annular photocatalytic slurry reactor [J].
Camera-Roda, Giovanni ;
Santarelli, Francesco ;
Panico, Mauro .
PHOTOCHEMICAL & PHOTOBIOLOGICAL SCIENCES, 2009, 8 (05) :712-718
[5]   Simulation and optimization of silicon thermal CVD through CFD integrating Taguchi method [J].
Cheng, W. T. ;
Li, H. C. ;
Huang, C. N. .
CHEMICAL ENGINEERING JOURNAL, 2008, 137 (03) :603-613
[6]  
Cheng YJ, 2006, IEEE T COMPON PACK T, V29, P39, DOI [10.1109/TCAPT.2005.848589, 10.1109/TCAPT.2006.]
[7]   A new approach to optimise an annular slurry photoreactor system for the degradation of Congo Red: Statistical analysis and modelling [J].
Chong, Meng Nan ;
Jin, Bo ;
Chow, Christopher W. K. ;
Saint, Chris P. .
CHEMICAL ENGINEERING JOURNAL, 2009, 152 (01) :158-166
[8]  
De Lasa H. I., 2005, PHOTOCATAL REACT ENG, DOI DOI 10.1007/0-387-27591-6_8
[9]  
Duran J. E., 2010, WATER SCI T IN PRESS
[10]   Computational Fluid Dynamics Modeling of Immobilized Photocatalytic Reactors for Water Treatment [J].
Duran, J. Esteban ;
Mohseni, Madjid ;
Taghipour, Fariborz .
AICHE JOURNAL, 2011, 57 (07) :1860-1872