Locking of Turing patterns in the chlorine dioxide-iodine-malonic acid reaction with one-dimensional spatial periodic forcing

被引:24
作者
Dolnik, Milos [1 ,2 ]
Bansagi, Tamas, Jr. [1 ,2 ]
Ansari, Sama [1 ,2 ]
Valent, Ivan [1 ,2 ,3 ]
Epstein, Irving R. [1 ,2 ]
机构
[1] Brandeis Univ, Dept Chem, Waltham, MA 02454 USA
[2] Brandeis Univ, Volen Ctr Complex Syst, Waltham, MA 02454 USA
[3] Comenius Univ, Fac Nat Sci, Dept Phys & Theoret Chem, Bratislava 84215, Slovakia
基金
美国国家科学基金会;
关键词
D O I
10.1039/c1cp20949c
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We use the photosensitive chlorine dioxide-iodine-malonic acid reaction-diffusion system to study wavenumber locking of Turing patterns with spatial periodic forcing. Wavenumber-locked stripe patterns are the typical resonant structures that labyrinthine patterns exhibit in response to one-dimensional forcing by illumination when images of stripes are projected on a working medium. Our experimental results reveal that segmented oblique, hexagonal and rectangular patterns can also be obtained. However, these two-dimensional resonant structures only develop in a relatively narrow range of forcing parameters, where the unforced stripe pattern is in close proximity to the domain of hexagonal patterns. Numerical simulations based on a model that incorporates the forcing by illumination using an additive term reproduce well the experimental observations. These findings confirm that additive one-dimensional forcing can generate a two-dimensional resonant response. However, such a response is considerably less robust than the effect of multiplicative forcing.
引用
收藏
页码:12578 / 12583
页数:6
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