Inhalation exposure of traffic police officers to polycyclic aromatic hydrocarbons (PAHs) during the winter in Beijing, China

被引:68
作者
Liu, Yanan
Tao, Shu [1 ]
Yang, Yifeng
Dou, Han
Yang, Yu
Coveney, Raymond M.
机构
[1] Peking Univ, Coll environm Sci, Lab Earth Surface Processes, Beijing 100871, Peoples R China
[2] Univ Missouri, Dept Geosci, Ctr Appl Environm Res, Kansas City, MO 64110 USA
基金
中国国家自然科学基金;
关键词
PAHs; exposure; police; car emission; risk;
D O I
10.1016/j.scitotenv.2007.05.008
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This study concerns the use of personal samplers to evaluate the exposure of traffic police to polycyclic aromatic hydrocarbons (PAHs) during the winter of 2005 in Beijing. We measured the samples collected for gas and particulate phases PAHs with the same technique used for an earlier study during the summer of 2004, and evaluated exposure risk based on the calculated benzo(a)pyrene equivalent concentrations (BaPeq) of both summer and winter. The mean exposure concentrations of gaseous and particulate phase PAHs in the winter are 4300 2900 ng/m(3) and 750 1000 ng/m(3), respectively, significantly higher than those measured simultaneously at control sites and also considerably higher than the values measured during the summer. The exposure PAH profiles for police and the control subjects are similar with predominant naphthalene in gaseous phase and dominant fluoranthene, pyrene, anthracene and naphthalene in particulate phase. Large daily variations occur both in summer and winter, because of the changes in the weather conditions especially wind speed and relative humidity which tend to disperse and scavenge PAHs in air. In the winter, the aver-age BaPeq value for traffic police is 82.1 ng/m(3), which is significantly higher than those for the control subjects and the national standard of 10 ng/m(3) for ambient air. Particulate phase PAHs contribute more than 90% of the total exposure risk in the winter. Annually, weighted-average probabilities of exceeding the national standard (10 ng/m(3)) are 69.3% and 20.6% for the police and the controls, respectively (c) 2007 Published by Elsevier B.V.
引用
收藏
页码:98 / 105
页数:8
相关论文
共 27 条
[1]  
AIZENBERG V, 1998, J AEROSOL SCI, V29, P1135
[2]  
[Anonymous], 2000, AIR QUAL GUID
[3]  
*BEIJ MUN GOV, 2004, BEIJ CIT PLANN 2004
[4]   Toxicity and genotoxicity of industrial soils polluted by polycyclic aromatic hydrocarbons (PAHs) [J].
Bispo, A ;
Jourdain, MJ ;
Jauzein, M .
ORGANIC GEOCHEMISTRY, 1999, 30 (8B) :947-952
[5]   Cancer risk assessment, indicators, and guidelines for polycyclic aromatic hydrocarbons in the ambient air [J].
Boström, CE ;
Gerde, P ;
Hanberg, A ;
Jernström, B ;
Johansson, C ;
Kyrklund, T ;
Rannug, A ;
Törnqvist, M ;
Victorin, K ;
Westerholm, R .
ENVIRONMENTAL HEALTH PERSPECTIVES, 2002, 110 :451-488
[6]   Chromosomal damage in peripheral blood lymphocytes of traffic policemen and taxi drivers exposed to urban air pollution [J].
Burgaz, S ;
Demircigil, GC ;
Karahalil, B ;
Karakaya, AE .
CHEMOSPHERE, 2002, 47 (01) :57-64
[7]  
*CHIN EPA, 1966, AMB AIR QUAL STAND G
[8]   Temporal trends, temperature dependence, and relative reactivity of atmospheric polycyclic aromatic hydrocarbons [J].
Dimashki, M ;
Lim, LH ;
Harrison, RM ;
Harrad, S .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2001, 35 (11) :2264-2267
[9]   Octanol-air partition coefficient as a predictor of partitioning of semi-volatile organic chemicals to aerosols [J].
Finizio, A ;
Mackay, D ;
Bidleman, T ;
Harner, T .
ATMOSPHERIC ENVIRONMENT, 1997, 31 (15) :2289-2296
[10]   Atmospheric bulk deposition of PAHs onto France: trends from urban to remote sites [J].
Garban, B ;
Blanchoud, H ;
Motelay-Massei, A ;
Chevreuil, M ;
Ollivon, D .
ATMOSPHERIC ENVIRONMENT, 2002, 36 (34) :5395-5403