Spontaneous emission of organic molecules embedded in a photonic crystal

被引:297
作者
Petrov, EP
Bogomolov, VN
Kalosha, II
Gaponenko, SV
机构
[1] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk 220072, BELARUS
[2] Russian Acad Sci, AF Ioffe Physicotech Inst, St Petersburg 194021, Russia
[3] Natl Acad Sci Belarus, Inst Atom & Mol Phys, Minsk 220072, BELARUS
关键词
D O I
10.1103/PhysRevLett.81.77
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report on modification of the spontaneous emission of dye molecules embedded in a three-dimensional solid-state photonic crystal exhibiting a stop band in the visible range. Molecules embedded in artificial opal filled with a polymer show a dip in the fluorescence spectrum and nonexponential spontaneous decay kinetics containing both accelerated and inhibited components compared to the dye fluorescence in a reference polymer matrix. Results are interpreted in terms of redistribution of the photon density of states in the photonic crystal.
引用
收藏
页码:77 / 80
页数:4
相关论文
共 40 条
[1]   Sum rule for modified spontaneous emission rates [J].
Barnett, SM ;
Loudon, R .
PHYSICAL REVIEW LETTERS, 1996, 77 (12) :2444-2446
[2]   Photonic band gaps in colloidal systems [J].
Biswas, R ;
Sigalas, MM ;
Subramania, G ;
Ho, KM .
PHYSICAL REVIEW B, 1998, 57 (07) :3701-3705
[3]   Photonic band gap in the visible range in a three-dimensional solid state lattice [J].
Bogomolov, VN ;
Gaponenko, SV ;
Kapitonov, AM ;
Prokofiev, AV ;
Ponyavina, AN ;
Silvanovich, NI ;
Samoilovich, SM .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 1996, 63 (06) :613-616
[4]   Photonic band gap phenomenon and optical properties of artificial opals [J].
Bogomolov, VN ;
Gaponenko, SV ;
Germanenko, IN ;
Kapitonov, AM ;
Petrov, EP ;
Gaponenko, NV ;
Prokofiev, AV ;
Ponyavina, AN ;
Silvanovich, NI ;
Samoilovich, SM .
PHYSICAL REVIEW E, 1997, 55 (06) :7619-7625
[5]  
BOLOTKO LM, 1973, J APPL SPECTROSC, V18, P714
[6]   SPONTANEOUS EMISSION IN THE OPTICAL MICROSCOPIC CAVITY [J].
DEMARTINI, F ;
MARROCCO, M ;
MATALONI, P ;
CRESCENTINI, L ;
LOUDON, R .
PHYSICAL REVIEW A, 1991, 43 (05) :2480-2497
[7]  
DEMARTINI F, 1987, PHYS REV LETT, V59, P2955, DOI 10.1103/PhysRevLett.59.2955
[8]  
Drexhage K. H., 1974, PROGR OPTICS, V12
[9]   CLASSICAL WAVE-PROPAGATION IN PERIODIC STRUCTURES - CERMET VERSUS NETWORK TOPOLOGY [J].
ECONOMOU, EN ;
SIGALAS, MM .
PHYSICAL REVIEW B, 1993, 48 (18) :13434-13438
[10]   FLUORESCENCE DECAY TIME DISTRIBUTION FOR POLAR DYE SOLUTIONS WITH TIME-DEPENDENT FLUORESCENT SHIFT [J].
GAKAMSKY, DM ;
GOLDIN, AA ;
PETROV, EP ;
RUBINOV, AN .
BIOPHYSICAL CHEMISTRY, 1992, 44 (01) :47-60