Observation of the simultaneous transport of Asian mineral dust aerosols with anthropogenic pollutants using a POPC during a long-lasting dust event in late spring 2014

被引:48
作者
Pan, Xiaole [1 ]
Uno, Itsushi [1 ]
Hara, Yukari [1 ]
Kuribayashi, Masatoshi [1 ]
Kobayashi, Hiroshi [2 ]
Sugimoto, Nobuo [3 ]
Yamamoto, Shigekazu [4 ]
Shimohara, Takaaki [4 ]
Wang, Zifa [5 ]
机构
[1] Kyushu Univ, Res Inst Appl Mech, Fukuoka 812, Japan
[2] Univ Yamanashi, Dept Ecosocial Syst Engn, Kofu, Yamanashi, Japan
[3] Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan
[4] Fukuoka Inst Hlth & Environm Sci, Fukuoka, Japan
[5] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing, Peoples R China
基金
日本学术振兴会;
关键词
dust aerosols; anthropogenic pollutants; depolarization ratio; East Asia; OPTICAL PARTICLE COUNTER; ACE-ASIA;
D O I
10.1002/2014GL062491
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
We observed a long-lasting dust event from 25 May to 2 June 2014, using a polarization optical particle counter (POPC). The transport of dust plumes over East Asia was verified on the basis of observations of Moderate Resolution Imaging Spectroradiometer, a lidar network, and surface synoptic observation stations. Mixing of dust and anthropogenic pollutants was investigated according to the variation in the depolarization ratio as a function of particle size. The nonsphericity of dust particles varied due to the impact of anthropogenic pollutants on their pathway. In the coarse mode, dust particles always had a clear nonspherical configuration, although large amounts of nitrate were also present. Supermicron particles are occasionally present in a spherical configuration, possibly due to the complex mixing of natural dust and anthropogenic particles. Statistically, similar to 64% of the total nitrate mass was deemed to be transported from outside of Japan due to a trapping effect in the dust plume.
引用
收藏
页码:1593 / 1598
页数:6
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