Influence of the synthesis atmosphere on NIR fluorescence behavior of Ce/Er co-doped bismuth glass through valence state changes of cerium

被引：5
作者：
Zhao, Guoying [1 ]
Xu, Lingzhi [1 ]
Jin, Wentian [1 ]
Song, Siyuan [1 ]
Hou, Jingshan [1 ]
Liu, Yufeng [1 ]
Guo, Yanyan [2 ]
Fang, Yongzheng [1 ]
Liao, Meisong [3 ]
Zou, Jun [3 ]
Hu, Lili [4 ]
机构：
[1] Shanghai Inst Technol, Sch Mat Sci & Engn, Shanghai 201418, Peoples R China
[2] Changchun Univ Sci & Technol, Coll Mat Sci & Engn, Changchun 130022, Jilin, Peoples R China
[3] Shanghai Inst Technol, Coll Sci, Shanghai 201418, Peoples R China
[4] Chinese Acad Sci, Key Lab Mat High Power Laser, Shanghai Inst Opt & Fine Mech, Shanghai 201800, Peoples R China
来源：
OPTICAL MATERIALS EXPRESS | 2018年 / 8卷 / 01期
基金：
中国国家自然科学基金;
关键词：
CEO2; THIN-FILMS; SPECTROSCOPIC PROPERTIES; PHOTOLUMINESCENCE PROPERTIES; TELLURITE GLASS; CE3+; LUMINESCENCE; ER3+; CE3+-CE4+; AMPLIFIER; PHOSPHOR;
D O I：
10.1364/OME.8.000030
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
This work investigates the near-infrared emission characteristics and energy transfer between erbium and cerium in bismuth glass by the reaction atmosphere process. The Er3+: 1.5 mu m emission can be successfully enhanced by performing a reduction conversion of Ce4+ -> Ce3+ using a reducing atmosphere. The discrepancies of the energy structure between Ce3+ and Ce4+ result in a contrasting sensitizing effect on Er3+: 1.5 mu m emission intensity and decay lifetime. The results show that a significant amount of Ce3+ is present in glasses prepared in a reducing atmosphere, whereas Ce4+ is the main species in an oxidizing atmosphere by means of absorption spectra and XPS curves. The reason for upconversion quenching is also discussed. (c) 2017 Optical Society of America under the terms of the OSA Open Access Publishing Agreement
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收藏
页码：30 / 40
页数：11
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