Methane Steam Reforming in Microchannel Reactors: Technical Challenges and Performances Benefits

被引：11

作者：

Grasso, Giacomo ^{[1
]}

Schaefer, Gerd ^{[2
]}

Schuurman, Yves ^{[1
]}

Mirodatos, Claude ^{[1
]}

机构：

[1] Univ Lyon 1, CNRS, UMR 5256, IRCELYON,Inst Rech Catalyse & Environm Lyon, F-69626 Villeurbanne, France

[2] Atotech Deutschland GmbH, D-10553 Berlin, Germany

来源：

TOPICS IN CATALYSIS | 2011年 / 54卷 / 13-15期

关键词：

Methane steam reforming; Microreactors; Microchannel reactors; Microstructured reactors; Brazing; Bonding; Laser welding; Nickel; Rhodium; MICROSTRUCTURED REACTORS; HEAT-TRANSFER; CATALYSTS; CONVERSION; HYDROGEN;

D O I：

10.1007/s11244-011-9707-9

中图分类号：

O69 [应用化学];

学科分类号：

081704 ;

摘要：

The steam reforming of methane was studied over microstructured platelets coated with catalysts and assembled as microreactors. Three different bonding procedures have been applied to assemble the microchannel platelets. The effect of the assembly procedure on the catalytic performance has been investigated for both nickel and rhodium based catalysts. The brazing technology leads, contrary to laser welding, to fully connected platelets resulting in a superior catalytic activity due to better heat transfer and gas flow distribution. Outstanding performances in term on hydrogen productivity and catalytic stability are obtained on the low temperature brazed system washcoated with a Rh-alumina catalyst.

引用

页码：859 / 865

页数：7

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