Tuning the Density of Zwitterionic Polymer Brushes on PET Fabrics by Aminolysis: Effect on Antifouling Performances

被引：18
作者：
Lorusso, Emanuela [1 ,2 ,3 ]
Ali, Wael [2 ,3 ,4 ]
Leniart, Michael [4 ]
Gebert, Beate [4 ]
Oberthuer, Markus [5 ]
Gutmann, Jochen S. [1 ,2 ,3 ,4 ]
机构：
[1] Deutsch Textilforsch Zentrum Nord West OP GmbH, D-47798 Krefeld, Germany
[2] Univ Duisburg Essen, Dept Phys Chem, D-45141 Essen, Germany
[3] Univ Duisburg Essen, Ctr Nanointegrat CENIDE, D-45141 Essen, Germany
[4] Deutsch Textilforsch Zentrum Nord West gGmbH, D-47798 Krefeld, Germany
[5] Hsch Angew Wissensch HAW Hamburg, Dept Design, D-22087 Hamburg, Germany
来源：
POLYMERS | 2020年 / 12卷 / 01期
关键词：
aminolysis; textiles; PET; functional coatings; polymer brushes; PROTEIN SURFACE INTERACTIONS; LUBRICANT-INFUSED SURFACES; POLY(ETHYLENE GLYCOL); POLYETHYLENE OXIDE; BIOFILMS; DESIGN; RESIST; POLY(ETHYLENE-TEREPHTHALATE); FUNCTIONALIZATION; NANOPARTICLES;
D O I：
10.3390/polym12010006
中图分类号：
O63 [高分子化学（高聚物）];
学科分类号：
070305 ; 080501 ; 081704 ;
摘要：
Here, we synthesize zwitterionic polymer brushes on polyester fabrics by atom transfer radical polymerization (ATRP) after a prefunctionalization step involving an aminolysis reaction with ethylenediamine. Aminolysis is an easy method to achieve homogeneous distributions of functional groups on polyester fibers (PET) fabrics. Varying the polymerization time and the prefunctionalization conditions of the reaction, it is possible to tune the amount of water retained over the surface and study its effect on protein adhesion. This study revealed that the polymerization time plays a major role in preventing protein adhesion on the PET surface.
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页数：14
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共 63 条
[31]   Atmospheric air-plasma treatments of polyester textile structures [J].
Leroux, F. ;
Perwuelz, A. ;
Campagne, C. ;
Behary, N. .
JOURNAL OF ADHESION SCIENCE AND TECHNOLOGY, 2006, 20 (09) :939-957
[32]   Bio-Click Chemistry: Enzymatic Functionalization of PEGylated Capsules for Targeting Applications [J].
Leung, Melissa K. M. ;
Hagemeyer, Christoph E. ;
Johnston, Angus P. R. ;
Gonzales, Catalina ;
Kamphuis, Marloes M. J. ;
Ardipradja, Katie ;
Such, Georgina K. ;
Peter, Karlheinz ;
Caruso, Frank .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2012, 51 (29) :7132-7136
[33]   Endocytic pH-Triggered Degradation of Nanoengineered Multilayer Capsules [J].
Liang, Kang ;
Such, Georgina K. ;
Johnston, Angus P. R. ;
Zhu, Zhiyuan ;
Ejima, Hirotaka ;
Richardson, Joseph J. ;
Cui, Jiwei ;
Caruso, Frank .
ADVANCED MATERIALS, 2014, 26 (12) :1901-1905
[34]   Hydrogel Functionalized Polyester Fabrics by UV-Induced Photopolymerization [J].
Lorusso, Emanuela ;
Ali, Wael ;
Hildebrandt, Marcus ;
Mayer-Gall, Thomas ;
Gutmann, Jochen S. .
POLYMERS, 2019, 11 (08)
[35]   Antibiofouling polymer interfaces: poly(ethylene glycol) and other promising candidates [J].
Lowe, Sean ;
O'Brien-Simpson, Neil M. ;
Connal, Luke A. .
POLYMER CHEMISTRY, 2015, 6 (02) :198-212
[36]   Non-fouling oligo(ethylene glycol)-functionalized polymer brushes synthesized by surface-initiated atom transfer radical polymerization [J].
Ma, HW ;
Hyun, JH ;
Stiller, P ;
Chilkoti, A .
ADVANCED MATERIALS, 2004, 16 (04) :338-+
[37]   Mechanisms of biofilm resistance to antimicrobial agents [J].
Mah, TFC ;
O'Toole, GA .
TRENDS IN MICROBIOLOGY, 2001, 9 (01) :34-39
[38]   Slippery Liquid-Infused Porous Surfaces that Prevent Microbial Surface Fouling and Kill Non-Adherent Pathogens in Surrounding Media: A Controlled Release Approach [J].
Manna, Uttam ;
Raman, Namrata ;
Welsh, Michael A. ;
Zayas-Gonzalez, Yashira M. ;
Blackwell, Helen E. ;
Palecek, Sean P. ;
Lynn, David M. .
ADVANCED FUNCTIONAL MATERIALS, 2016, 26 (21) :3599-3611
[39]   Polyvinylamine modified polyester fibers - innovative textiles for the removal of chromate from contaminated groundwater [J].
Mayer-Gall, Thomas ;
Opwis, Klaus ;
Gutmann, Jochen S. .
JOURNAL OF MATERIALS CHEMISTRY A, 2015, 3 (01) :386-394
[40]   Study of oxygen plasma pre-treatment of polyester fabric for improved polypyrrole adhesion [J].
Mehmood, Tariq ;
Kaynak, Akif ;
Dai, Xiujuan J. ;
Kouzani, Abbas ;
Magniez, Kevin ;
de Celis, David Rubin ;
Hurren, Christopher J. ;
du Plessis, Johan .
MATERIALS CHEMISTRY AND PHYSICS, 2014, 143 (02) :668-675
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