Co-assembly of photosystem II/reduced graphene oxide multilayered biohybrid films for enhanced photocurrent

被引:51
作者
Cai, Peng [1 ]
Feng, Xiyun [1 ]
Fei, Jinbo [1 ]
Li, Guangle [1 ]
Li, Jiao [1 ,2 ]
Huang, Jianguo [2 ]
Li, Junbai [1 ]
机构
[1] Chinese Acad Sci, BNLMS, CAS Key Lab Colloid Interface & Chem Thermodynam, Inst Chem, Beijing 100190, Peoples R China
[2] Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China
基金
中国国家自然科学基金;
关键词
PHOTO-BIOELECTROCHEMICAL CELLS; ELECTRON-TRANSFER; WATER OXIDATION; SOLAR; GENERATION; ARCHITECTURES; ORGANIZATION; MEMBRANES;
D O I
10.1039/c5nr02322j
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A new type of biohybrid photo-electrochemical cell was fabricated by layer-by-layer assembly of photosystem II and reduced graphene oxide. We demonstrate that the photocurrent in the direct electron transfer is enhanced about two fold with improved stability. The assembly strategy without any cross-linker or additional electron mediators makes the cell fabrication and operation much simpler as compared to previous approaches. This work may open new routes for the construction of solar energy conversion systems based on photoactive proteins and graphene materials.
引用
收藏
页码:10908 / 10911
页数:4
相关论文
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