Oxidation Processes and Involved Chemical Reactions of Corrosion-Resistant Alloys in Supercritical Water

被引：29
作者：
Guo, Shuwei [1 ]
Xu, Donghai [1 ]
Wei, Ning [1 ]
Wang, Yuzhen [2 ]
Chen, Gang [3 ]
Wang, Shuzhong [1 ]
机构：
[1] Xi An Jiao Tong Univ, Sch Energy & Power Engn, Minist Educ, Key Lab Thermofluid Sci & Engn, Xian 710049, Shaanxi, Peoples R China
[2] Xian Univ Technol, Xian 710048, Shaanxi, Peoples R China
[3] Shaanxi Coal & Chem Technol Inst Co Ltd, Xian 710070, Shaanxi, Peoples R China
来源：
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH | 2020年 / 59卷 / 22期
基金：
中国国家自然科学基金;
关键词：
FERRITIC-MARTENSITIC STEEL; 316L STAINLESS-STEEL; NI-BASE ALLOYS; HIGH-TEMPERATURE WATER; DISSOLVED-OXYGEN; OXIDE SCALES; CRACKING SUSCEPTIBILITY; EXPOSURE TEMPERATURE; CHROMIA EVAPORATION; AUSTENITIC ALLOYS;
D O I：
10.1021/acs.iecr.0c01394
中图分类号：
TQ [化学工业];
学科分类号：
0817 ;
摘要：
Corrosion continues to be a major challenge in developing supercritical water-cooled reactor and supercritical water oxidation systems. Corrosion behaviors of candidate alloy materials used in these environments are significantly affected by the properties of oxides formed on alloy surfaces. This work presents a comprehensive review of the oxidation processes and involved chemical reactions of corrosion-resistant alloys in supercritical water. The oxidation process of an alloy in supercritical water is proposed to have two stages, and chemical reactions at these two stages are described in detail. The transitions of Cr/Ni/Fe oxides and the formation mechanism of oxide film are analyzed comprehensively. Moreover, the diffusion property, protection effect, and stability of oxides in supercritical water are summarized systematically.
引用
收藏
页码：10278 / 10288
页数：11
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