Seasonal variation of PM10-bound PAHs in the atmosphere of Xiamen, China

被引：111

作者：

Hong, HuaSheng ^{[1
]}

Yin, HongLing ^{[1
]}

Wang, XinHong ^{[1
]}

Ye, CuiXing ^{[1
]}

机构：

[1] Xiamen Univ, State Key Lab Marine Environm Sci, Fujian 361005, Peoples R China

来源：

ATMOSPHERIC RESEARCH | 2007年 / 85卷 / 3-4期

关键词：

polycyclic aromatic hydrocarbons; aerosol; seasonal variation; source identification;

D O I：

10.1016/j.atmosres.2007.03.004

中图分类号：

P4 [大气科学（气象学）];

学科分类号：

0706 ; 070601 ;

摘要：

PM10 samples from a garden site (site A), an industrial-traffic intersection (site B), a residential site (site C) and an island site (site D) were collected at December 21-29, 2004; March 18-22, 2005; July 4-13, 2005 and October 24-28, 2005 in Xiamen. 15 priority PAHs compounds were analyzed by using a gas chromatograph/mass spectrometer (GUMS). The abundance and origin of 3 PAHs are discussed to reveal seasonal variations in Xiamen air quality. Average concentrations of Sigma 15PAHs were 17.5 ng/m(3), 3.7 ng/m(3), 32.6 ng/m(3) and 10.5 ng/m(3) from spring to winter with the highest value in autumn. The dominant PAHs components in every season were low and middle molecular weight PAHs including phenanthrene, pyrene, fluoranthene and chrysene. Diagnostic ratios and PCA analysis identified the main sources of particle bound PAHs: mainly from both gasoline and diesel vehicles exhaust, with some contribution from coal combustion, industry emission and cooking sources. (C) 2007 Published by Elsevier B.V.

引用

页码：429 / 441

页数：13

共 61 条

[1] METHODS FOR DETECTING CARCINOGENS AND MUTAGENS WITH SALMONELLA-MAMMALIAN-MICROSOME MUTAGENICITY TEST [J].

AMES, BN ;

MCCANN, J ;

YAMASAKI, E .

MUTATION RESEARCH, 1975, 31 (06) :347-363

[2]

[Anonymous], [No title captured]

[3]

[Anonymous], 1979, POLYNUCLEAR AROMATIC

[4] CORRELATIONS BETWEEN 15 POLYCYCLIC AROMATIC-HYDROCARBONS (PAH) AND THE MUTAGENICITY OF THE TOTAL PAH FRACTION IN AMBIENT AIR PARTICLES IN LA-SPEZIA (ITALY) [J].

BARALE, R ;

GIROMINI, L ;

GHELARDINI, G ;

SCAPOLI, C ;

LOPRIENO, N ;

PALA, M ;

VALERIO, F ;

BARRAI, I .

MUTATION RESEARCH, 1991, 249 (01) :227-241

[5] Extractable organic matter in PM10 from LiWan district of Guangzhou city, PR China [J].

Bi, XH ;

Sheng, GY ;

Peng, PA ;

Zhang, ZQ ;

Fu, HM .

SCIENCE OF THE TOTAL ENVIRONMENT, 2002, 300 (1-3) :213-228

[6] A wintertime study of PAHs in fine and coarse aerosols in Sao Paulo city, Brazil [J].

Bourotte, C ;

Forti, MC ;

Taniguchi, S ;

Bícego, MC ;

Lotufo, PA .

ATMOSPHERIC ENVIRONMENT, 2005, 39 (21) :3799-3811

[7] Polycyclic aromatic hydrocarbons in the urban atmospheric particulate matter in the city of Naples (Italy) [J].

Caricchia, AM ;

Chiavarini, S ;

Pezza, M .

ATMOSPHERIC ENVIRONMENT, 1999, 33 (23) :3731-3738

[8] Atmospheric polycyclic aromatic hydrocarbons (PAHs) in Asia: A review from 1999 to 2004 [J].

Chang, Kuan-Foo ;

Fang, Guor-Cheng ;

Chen, Jhy-Cherng ;

Wu, Yuh-Shen .

ENVIRONMENTAL POLLUTION, 2006, 142 (03) :388-396

[9] A comparison of temporal variation of particle-bound polycyclic aromatic hydrocarbons (pPAHs) concentration in different urban environments: Tokyo, Japan, and Bangkok, Thailand [J].

Chetwittayachan, T ;

Shimazaki, D ;

Yamamoto, K .

ATMOSPHERIC ENVIRONMENT, 2002, 36 (12) :2027-2037

[10]

*CHIN ENV PROT BUR, 1996, GB3095

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