Progress and Perspectives of Organosulfur for Lithium-Sulfur Batteries

被引：118
作者：
Pan, Zhiyong [1 ]
Brett, Dan J. L. [2 ]
He, Guanjie [1 ,2 ,3 ]
Parkin, Ivan P. [1 ]
机构：
[1] UCL, Dept Chem, Christopher Ingold Lab, 20 Gordon St, London WC1H 0AJ, England
[2] UCL, Dept Chem Engn, Electrochem Innovat Lab, London WC1E 7JE, England
[3] Univ Lincoln, Sch Chem, Joseph Banks Labs, Green Lane, Lincoln LN6 7DL, England
来源：
ADVANCED ENERGY MATERIALS | 2022年 / 12卷 / 08期
基金：
英国工程与自然科学研究理事会;
关键词：
binders; cathodes; electrolytes; interlayers; lithium-sulfur batteries; organosulfur; CATHODE MATERIALS; ELEMENTAL SULFUR; PERFORMANCE; COMPOSITE; POLYACRYLONITRILE; POLYSULFIDES; ELECTROLYTE; ADDITIVES; CHEMISTRY; STORAGE;
D O I：
10.1002/aenm.202103483
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Lithium-sulfur batteries (LSBs) with high theoretical capacity are regarded as the most promising candidates for next-generation energy storage systems. However, the low conductivity, high volume change, and shuttle effect need to be addressed before the commercialization of LSBs. Organosulfur with covalent C-S bonds can solve these problems when applied as different components of LSBs. Recent advances of application of organosulfur as cathodes, electrolytes, interlayers, and binders in LSBs are reviewed. Finally, the prospects for organosulfur are proposed from both the perspectives of mechanism understanding and practical applications.
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页数：18
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