Global and Local Impacts of Delayed Mercury Mitigation Efforts

被引:24
作者
Angot, Helene [1 ]
Hoffman, Nicholas [2 ]
Giang, Amanda [1 ,3 ]
Thackray, Colin P. [4 ]
Hendricks, Ashley N. [5 ]
Urban, Noel R. [5 ]
Selin, Noelle E. [1 ,2 ]
机构
[1] MIT, Inst Data Syst & Soc, 77 Massachusetts Ave, Cambridge, MA 02139 USA
[2] MIT, Dept Earth Atmospher & Planetary Sci, Cambridge, MA 02139 USA
[3] Univ British Columbia, Inst Resources Environm & Sustainabil, Vancouver, BC V6T 1Z4, Canada
[4] Harvard Univ, Harvard John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA
[5] Michigan Technol Univ, Dept Civil & Environm Engn, Houghton, MI 49931 USA
基金
美国国家科学基金会;
关键词
PARTICULATE MERCURY; MODEL; EMISSIONS; POLLUTION; FISH; BIOACCUMULATION; DEPOSITION; ATMOSPHERE; EXPOSURE; CLIMATE;
D O I
10.1021/acs.est.8b04542
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Mercury (Hg) is emitted to air by natural and anthropogenic sources, transports and deposits globally, and bioaccumulates to toxic levels in food webs. It is addressed under the global 2017 Minamata Convention, for which periodic effectiveness evaluation is required. Previous analyses have estimated the impact of different regulatory strategies for future mercury deposition. However, analyses using atmospheric models traditionally hold legacy emissions (recycling of previously deposited Hg) constant, and do not account for their possible future growth. Here, using an integrated modeling approach, we investigate how delays in implementing emissions reductions and the associated growing legacy reservoir affect deposition fluxes to ecosystems in different global regions. Assuming nearly constant yearly emissions relative to 2010, each 5-year delay in peak emissions defers by additional extra ca. 4 years the return to year 2010 global deposition. On a global average, each 5-year delay leads to a 14% decrease in policy impacts on local-scale Hg deposition. We also investigate the response of fish contamination in remote lakes to delayed action. We quantify the consequences of delay for limiting the Hg burden of future generations and show that traditional analyses of policy impacts provide best-case estimates.
引用
收藏
页码:12968 / 12977
页数:10
相关论文
共 82 条
  • [1] Climate and productivity affect total mercury concentration and bioaccumulation rate of fish along a spatial gradient of subarctic lakes
    Ahonen, Salla A.
    Hayden, Brian
    Leppanen, Jaakko J.
    Kahilainen, Kimmo K.
    [J]. SCIENCE OF THE TOTAL ENVIRONMENT, 2018, 637 : 1586 - 1596
  • [2] AMAP/UNEP, 2013, TECHN BACKGR REP GLO, P263
  • [3] Gas-particle partitioning of atmospheric Hg(II) and its effect on global mercury deposition
    Amos, H. M.
    Jacob, D. J.
    Holmes, C. D.
    Fisher, J. A.
    Wang, Q.
    Yantosca, R. M.
    Corbitt, E. S.
    Galarneau, E.
    Rutter, A. P.
    Gustin, M. S.
    Steffen, A.
    Schauer, J. J.
    Graydon, J. A.
    St Louis, V. L.
    Talbot, R. W.
    Edgerton, E. S.
    Zhang, Y.
    Sunderland, E. M.
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2012, 12 (01) : 591 - 603
  • [4] Observational and Modeling Constraints on Global Anthropogenic Enrichment of Mercury
    Amos, Helen M.
    Sonke, Jeroen E.
    Obrist, Daniel
    Robins, Nicholas
    Hagan, Nicole
    Horowitz, Hannah M.
    Mason, Robert P.
    Witt, Melanie
    Hedgecock, Ian M.
    Corbitt, Elizabeth S.
    Sunderland, Elsie M.
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2015, 49 (07) : 4036 - 4047
  • [5] Global Biogeochemical Implications of Mercury Discharges from Rivers and Sediment Burial
    Amos, Helen M.
    Jacob, Daniel J.
    Kocman, David
    Horowitz, Hannah M.
    Zhang, Yanxu
    Dutkiewicz, Stephanie
    Horvat, Milena
    Corbitt, Elizabeth S.
    Krabbenhoft, David P.
    Sunderland, Elsie M.
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2014, 48 (16) : 9514 - 9522
  • [6] Legacy impacts of all-time anthropogenic emissions on the global mercury cycle
    Amos, Helen M.
    Jacob, Daniel J.
    Streets, David G.
    Sunderland, Elsie M.
    [J]. GLOBAL BIOGEOCHEMICAL CYCLES, 2013, 27 (02) : 410 - 421
  • [7] Meeting Minamata: Cost-effective compliance options for atmospheric mercury control in Chinese coal-fired power plants
    Ancora, Maria Pia
    Zhang, Lei
    Wang, Shuxiao
    Schreifels, Jeremy J.
    Hao, Jiming
    [J]. ENERGY POLICY, 2016, 88 : 485 - 494
  • [8] New clues on the contribution of Earth's volcanism to the global mercury cycle
    Bagnato, E.
    Aiuppa, A.
    Parello, F.
    Allard, P.
    Shinohara, H.
    Liuzzo, M.
    Giudice, G.
    [J]. BULLETIN OF VOLCANOLOGY, 2011, 73 (05) : 497 - 510
  • [9] Dietary uptake models used for modeling the bioaccumulation of organic contaminants in fish
    Barber, M. Craig
    [J]. ENVIRONMENTAL TOXICOLOGY AND CHEMISTRY, 2008, 27 (04) : 755 - 777
  • [10] Ice Core Perspective on Mercury Pollution during the Past 600 Years
    Beal, Samuel A.
    Osterberg, Erich C.
    Zdanowicz, Christian M.
    Fisher, David A.
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2015, 49 (13) : 7641 - 7647