Strain dependent defect mediated ferromagnetism in Mn-doped and undoped ZnO thin films

被引:21
作者
Schoofs, Frank [1 ]
Fix, Thomas [1 ]
Hakimi, Ali M. H. R. [1 ]
Dhesi, Sarnjeet S. [2 ]
van der Laan, Gerrit [2 ]
Cavill, Stuart A. [2 ]
Langridge, Sean [3 ]
MacManus-Driscoll, Judith L. [1 ]
Blamire, Mark G. [1 ]
机构
[1] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB2 3QZ, England
[2] Diamond Light Source, Didcot OX11 0DE, Oxon, England
[3] Rutherford Appleton Lab, Sci & Technol Facil Council, Didcot OX11 0QX, Oxon, England
基金
英国工程与自然科学研究理事会;
关键词
TEMPERATURE FERROMAGNETISM; ABSORPTION-SPECTRA;
D O I
10.1063/1.3455856
中图分类号
O59 [应用物理学];
学科分类号
摘要
The structural and magnetic properties of pulsed laser deposited zinc oxide thin films have been investigated. Room temperature ferromagnetism is present in undoped as well as Mn-doped films. The saturation magnetization of the thin films reveals a dependence on both the composition and the out of plane lattice parameter. X-ray magnetic circular dichroism down to 2 K reveals a purely paramagnetic contribution from the Mn in Mn:ZnO films. We conclude that the observed ferromagnetism arises entirely from intrinsic defects in the ZnO which can be varied by manipulation of the lattice parameter. (C) 2010 American Institute of Physics. [doi: 10.1063/1.3455856]
引用
收藏
页数:5
相关论文
共 32 条
[1]   Paramagnetism of the Co sublattice in ferromagnetic Zn1-xCoxO films [J].
Barla, A. ;
Schmerber, G. ;
Beaurepaire, E. ;
Dinia, A. ;
Bieber, H. ;
Colis, S. ;
Scheurer, F. ;
Kappler, J-P. ;
Imperia, P. ;
Nolting, F. ;
Wilhelm, F. ;
Rogalev, A. ;
Mueller, D. ;
Grob, J. J. .
PHYSICAL REVIEW B, 2007, 76 (12)
[2]   Enhancement of ferroelectricity in strained BaTiO3 thin films [J].
Choi, KJ ;
Biegalski, M ;
Li, YL ;
Sharan, A ;
Schubert, J ;
Uecker, R ;
Reiche, P ;
Chen, YB ;
Pan, XQ ;
Gopalan, V ;
Chen, LQ ;
Schlom, DG ;
Eom, CB .
SCIENCE, 2004, 306 (5698) :1005-1009
[3]   Dilute magnetic oxides [J].
Coey, J. M. D. .
CURRENT OPINION IN SOLID STATE & MATERIALS SCIENCE, 2006, 10 (02) :83-92
[4]   Structural, chemical and magnetic investigations of polycrystalline Zn1-xMnxO [J].
Deshmukh, Alka V. ;
Patil, S. I. ;
Yusuf, S. M. ;
Rajarajan, A. K. ;
Lalla, N. P. .
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS, 2010, 322 (05) :536-541
[5]   Zener model description of ferromagnetism in zinc-blende magnetic semiconductors [J].
Dietl, T ;
Ohno, H ;
Matsukura, F ;
Cibert, J ;
Ferrand, D .
SCIENCE, 2000, 287 (5455) :1019-1022
[6]   Surface effects in Mn L3,2 x-ray absorption spectra from (Ga,Mn)As [J].
Edmonds, KW ;
Farley, NRS ;
Campion, RP ;
Foxon, CT ;
Gallagher, BL ;
Johal, TK ;
van der Laan, G ;
MacKenzie, M ;
Chapman, JN ;
Arenholz, E .
APPLIED PHYSICS LETTERS, 2004, 84 (20) :4065-4067
[7]   Magnetic properties of sol-gel-derived doped ZnO as a potential ferromagnetic semiconductor: a synchrotron-based study [J].
Farley, N. R. S. ;
Edmonds, K. W. ;
Freeman, A. A. ;
van der Laan, G. ;
Staddon, C. R. ;
Gregory, D. H. ;
Gallagher, B. L. .
NEW JOURNAL OF PHYSICS, 2008, 10
[8]   Magnetic and electric phase control in epitaxial EuTiO3 from first principles [J].
Fennie, Craig J. ;
Rabe, Karin M. .
PHYSICAL REVIEW LETTERS, 2006, 97 (26)
[9]   Ferromagnetism in Co-doped (La,Sr)TiO3 [J].
Fix, T. ;
Liberati, M. ;
Aubriet, H. ;
Sahonta, S-L ;
Bali, R. ;
Becker, C. ;
Ruch, D. ;
MacManus-Driscoll, J. L. ;
Arenholz, E. ;
Blamire, M. G. .
NEW JOURNAL OF PHYSICS, 2009, 11
[10]   Magnetic properties of mn-doped ZnO [J].
Fukumura, T ;
Jin, ZW ;
Kawasaki, M ;
Shono, T ;
Hasegawa, T ;
Koshihara, S ;
Koinuma, H .
APPLIED PHYSICS LETTERS, 2001, 78 (07) :958-960